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WO2010003968A3 - Verfahren und vorrichtung zur herstellung von teerarmem synthesegas aus biomasse - Google Patents

Verfahren und vorrichtung zur herstellung von teerarmem synthesegas aus biomasse Download PDF

Info

Publication number
WO2010003968A3
WO2010003968A3 PCT/EP2009/058638 EP2009058638W WO2010003968A3 WO 2010003968 A3 WO2010003968 A3 WO 2010003968A3 EP 2009058638 W EP2009058638 W EP 2009058638W WO 2010003968 A3 WO2010003968 A3 WO 2010003968A3
Authority
WO
WIPO (PCT)
Prior art keywords
synthesis gas
tar
biomass
fluidized bed
bed reactor
Prior art date
Application number
PCT/EP2009/058638
Other languages
English (en)
French (fr)
Other versions
WO2010003968A2 (de
Inventor
Karl-Heinz Tetzlaff
Original Assignee
Karl-Heinz Tetzlaff
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Karl-Heinz Tetzlaff filed Critical Karl-Heinz Tetzlaff
Priority to EP09780289A priority Critical patent/EP2303995A2/de
Priority to CN200980126921XA priority patent/CN102089409A/zh
Priority to CA2739270A priority patent/CA2739270A1/en
Priority to BRPI0915559A priority patent/BRPI0915559A2/pt
Priority to US13/003,171 priority patent/US9011724B2/en
Priority to UAA201100221A priority patent/UA108981C2/en
Priority to RU2011104191/05A priority patent/RU2516533C2/ru
Priority to JP2011517149A priority patent/JP5731379B2/ja
Publication of WO2010003968A2 publication Critical patent/WO2010003968A2/de
Publication of WO2010003968A3 publication Critical patent/WO2010003968A3/de

Links

Classifications

    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J3/00—Production of combustible gases containing carbon monoxide from solid carbonaceous fuels
    • C10J3/58—Production of combustible gases containing carbon monoxide from solid carbonaceous fuels combined with pre-distillation of the fuel
    • C10J3/60—Processes
    • C10J3/64—Processes with decomposition of the distillation products
    • C10J3/66—Processes with decomposition of the distillation products by introducing them into the gasification zone
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10B—DESTRUCTIVE DISTILLATION OF CARBONACEOUS MATERIALS FOR PRODUCTION OF GAS, COKE, TAR, OR SIMILAR MATERIALS
    • C10B53/00—Destructive distillation, specially adapted for particular solid raw materials or solid raw materials in special form
    • C10B53/02—Destructive distillation, specially adapted for particular solid raw materials or solid raw materials in special form of cellulose-containing material
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J3/00—Production of combustible gases containing carbon monoxide from solid carbonaceous fuels
    • C10J3/46—Gasification of granular or pulverulent flues in suspension
    • C10J3/48—Apparatus; Plants
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J3/00—Production of combustible gases containing carbon monoxide from solid carbonaceous fuels
    • C10J3/46—Gasification of granular or pulverulent flues in suspension
    • C10J3/48—Apparatus; Plants
    • C10J3/482—Gasifiers with stationary fluidised bed
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J3/00—Production of combustible gases containing carbon monoxide from solid carbonaceous fuels
    • C10J3/72—Other features
    • C10J3/721—Multistage gasification, e.g. plural parallel or serial gasification stages
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/09—Details of the feed, e.g. feeding of spent catalyst, inert gas or halogens
    • C10J2300/0903—Feed preparation
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/09—Details of the feed, e.g. feeding of spent catalyst, inert gas or halogens
    • C10J2300/0903—Feed preparation
    • C10J2300/0909—Drying
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/09—Details of the feed, e.g. feeding of spent catalyst, inert gas or halogens
    • C10J2300/0983—Additives
    • C10J2300/0986—Catalysts
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10J—PRODUCTION OF PRODUCER GAS, WATER-GAS, SYNTHESIS GAS FROM SOLID CARBONACEOUS MATERIAL, OR MIXTURES CONTAINING THESE GASES; CARBURETTING AIR OR OTHER GASES
    • C10J2300/00—Details of gasification processes
    • C10J2300/12—Heating the gasifier
    • C10J2300/123—Heating the gasifier by electromagnetic waves, e.g. microwaves
    • C10J2300/1238—Heating the gasifier by electromagnetic waves, e.g. microwaves by plasma
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E50/00—Technologies for the production of fuel of non-fossil origin
    • Y02E50/10—Biofuels, e.g. bio-diesel

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Organic Chemistry (AREA)
  • Combustion & Propulsion (AREA)
  • Materials Engineering (AREA)
  • Processing Of Solid Wastes (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Devices And Processes Conducted In The Presence Of Fluids And Solid Particles (AREA)
  • Hydrogen, Water And Hydrids (AREA)
  • Production Of Liquid Hydrocarbon Mixture For Refining Petroleum (AREA)
  • Industrial Gases (AREA)

Abstract

Verfahren zur Erzeugung von Synthesegas aus Biomasse weisen einen hohen Teergehalt auf oder benötigen Temperaturen bei denen die Asche glasartig aufschmilzt und daher nicht als Mineraldünger verwendbar ist. Der Erfindung liegt die Aufgabe zugrunde, diese Nachteile zu vermeiden und ein hochwertiges Synthesegas mit einem hohen Wirkungsgrad herzustellen. Mit dem erfindungsgemäßen Verfahren wird der Teergehalt im Synthesegas (15a) dadurch abgesenkt, dass die Biomasse (1) in einem Wirbelschichtreaktor (3) in Pyrolysekoks und Pyrolysegas gespalten, und beide mindestens einem weiteren Wirbelschichtreaktor (11) zugeführt werden, wobei Teere bei höherer Temperatur an dem weitgehend teerfreien Pyrolysekoks katalytisch gespalten werden, ohne dass der Ascheschmelzpunkt überschritten wird. Das erfindungsgemäße Verfahren ermöglicht die Herstellung von weitgehend teerfreiem Synthesegas.
PCT/EP2009/058638 2008-07-08 2009-07-07 Verfahren und vorrichtung zur herstellung von teerarmem synthesegas aus biomasse WO2010003968A2 (de)

Priority Applications (8)

Application Number Priority Date Filing Date Title
EP09780289A EP2303995A2 (de) 2008-07-08 2009-07-07 Verfahren und vorrichtung zur herstellung von teerarmem synthesegas aus biomasse
CN200980126921XA CN102089409A (zh) 2008-07-08 2009-07-07 由生物质制造低焦油合成气的方法及装置
CA2739270A CA2739270A1 (en) 2008-07-08 2009-07-07 Method and device for producing low-tar synthesis gas from biomass
BRPI0915559A BRPI0915559A2 (pt) 2008-07-08 2009-07-07 processo e dispositivo para a produção, a partir de biomassa, de gás de síntese com reduzido teor de alcatrão
US13/003,171 US9011724B2 (en) 2008-07-08 2009-07-07 Method and device for producing low-tar synthesis gas from biomass
UAA201100221A UA108981C2 (en) 2008-07-08 2009-07-07 METHOD AND INSTALLATION FOR OBTAINING SYNTHESIS GAS WITH A SMALL CONTENT OF RESIN FROM BIOMASS
RU2011104191/05A RU2516533C2 (ru) 2008-07-08 2009-07-07 Способ и устройство для получения синтез-газа с низким содержанием смол из биомассы
JP2011517149A JP5731379B2 (ja) 2008-07-08 2009-07-07 バイオマスから低タール合成ガスを製造する方法および装置

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
DE102008032166A DE102008032166A1 (de) 2008-07-08 2008-07-08 Verfahren und Vorrichtung zur Herstellung von teerfreiem Synthesgas aus Biomasse
DE102008032166.4 2008-07-08

Publications (2)

Publication Number Publication Date
WO2010003968A2 WO2010003968A2 (de) 2010-01-14
WO2010003968A3 true WO2010003968A3 (de) 2010-04-08

Family

ID=41382059

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/EP2009/058638 WO2010003968A2 (de) 2008-07-08 2009-07-07 Verfahren und vorrichtung zur herstellung von teerarmem synthesegas aus biomasse

Country Status (12)

Country Link
US (1) US9011724B2 (de)
EP (1) EP2303995A2 (de)
JP (2) JP5731379B2 (de)
KR (1) KR20110052604A (de)
CN (1) CN102089409A (de)
BR (1) BRPI0915559A2 (de)
CA (1) CA2739270A1 (de)
DE (1) DE102008032166A1 (de)
RU (1) RU2516533C2 (de)
TW (1) TWI410487B (de)
UA (1) UA108981C2 (de)
WO (1) WO2010003968A2 (de)

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TWI410487B (zh) 2013-10-01
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JP5731379B2 (ja) 2015-06-10
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TW201009066A (en) 2010-03-01
US20120091395A1 (en) 2012-04-19
WO2010003968A2 (de) 2010-01-14
UA108981C2 (en) 2015-07-10
JP2015025145A (ja) 2015-02-05
CA2739270A1 (en) 2010-01-14
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