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Atmosphere, Volume 15, Issue 12 (December 2024) – 102 articles

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18 pages, 3070 KiB  
Article
Assessing the Effects of Wheat Planting on Groundwater Under Climate Change: A Quantitative Adaptive Sliding Window Detection Strategy
by Lingling Fan, Shi Chen, Lang Xia, Yan Zha and Peng Yang
Atmosphere 2024, 15(12), 1501; https://doi.org/10.3390/atmos15121501 - 16 Dec 2024
Abstract
Climate change has led to changes in precipitation patterns, exacerbating the overextraction of groundwater for wheat irrigation. Although many studies have examined the effects of wheat cultivation on groundwater storage (GWS), few studies have directly assessed the effects of wheat planting on GWS. [...] Read more.
Climate change has led to changes in precipitation patterns, exacerbating the overextraction of groundwater for wheat irrigation. Although many studies have examined the effects of wheat cultivation on groundwater storage (GWS), few studies have directly assessed the effects of wheat planting on GWS. We proposed a wheat subsiding effect detection (WSED) strategy using time-series remote sensing image to assess the effect of wheat area on GWS across China. The subsiding magnitude of the WSED is calculated as the GWS difference between the wheat area and adjacent nonwheat area in the self-adaptive moving window (the size and position of the sliding window can be automatically adjusted based on the characteristics of the data at the central pixel location). The effects of the wheat area on groundwater storage differ greatly among the change types of wheat area and planting regionalization, characterized by the strong subsiding effect in the wheat stable area, gain area, and Huanghuaihai zone (HWW, the most important wheat-producing region in China mainly includes the provinces and municipalities of Beijing, Tianjin, Henan, Hebei, Shandong, Anhui, and Jiangsu). Nearly 80% of the wheat area in the stable and gain regions had lower groundwater depth than nonwheat areas with significant differences (p < 0.05), resulting in a clear declining groundwater trend of approximately −1 cm/year. This study provides quantitative evidence for the effects of wheat planting on GWS regarding agricultural production and climate change adaptations. Full article
(This article belongs to the Special Issue Observation of Climate Change and Cropland with Satellite Data)
21 pages, 3487 KiB  
Article
Spatial and Temporal Distribution of CO2 and Thermal Comfort Conditions in a Day Care Center
by José María Moral Luque, José Luis Sánchez Jiménez and Manuel Ruiz de Adana
Atmosphere 2024, 15(12), 1500; https://doi.org/10.3390/atmos15121500 - 16 Dec 2024
Abstract
Finding the balance between CO2 concentration and thermal comfort is very important during the heating season in a daycare classroom due to the impact it has on children’s health. Air treatment systems together with outdoor hygrothermal conditions are decisive in finding this [...] Read more.
Finding the balance between CO2 concentration and thermal comfort is very important during the heating season in a daycare classroom due to the impact it has on children’s health. Air treatment systems together with outdoor hygrothermal conditions are decisive in finding this balance. The objective of this work is to evaluate the impact that three air treatment systems, ventilation, conditioning, and air cleaning, have on thermal comfort and CO2 concentration in the two breathing planes defined by the occupants of a daycare classroom. Eight experimental tests were carried out, using different combinations of air systems. Temperature, relative humidity, and CO2 concentration are measured at eight points in the classroom: four in the children’s breathing plane (0.75 m) and the other four in that of an adult (1.7 m). The results show, on the one hand, that the ventilation or conditioning systems improve the indoor CO2 concentration in the two planes, equalizing it in the two planes and, on the other hand, that the sensation of cold is greater in the children’s breathing plane than in the adult’s breathing plane in all the experimental tests studied. Full article
18 pages, 7604 KiB  
Article
Driving Force of Meteorology and Emissions on PM2.5 Concentration in Major Urban Agglomerations in China
by Jiqiang Niu, Hongrui Li, Xiaoyong Liu, Hao Lin, Peng Zhou and Xuan Zhu
Atmosphere 2024, 15(12), 1499; https://doi.org/10.3390/atmos15121499 - 16 Dec 2024
Abstract
Air pollution is influenced by a combination of pollutant emissions and meteorological conditions. Anthropogenic emissions and meteorological conditions are the two main causes of atmospheric pollution, and the contribution of meteorology and emissions to the reduction of PM2.5 concentrations across the country [...] Read more.
Air pollution is influenced by a combination of pollutant emissions and meteorological conditions. Anthropogenic emissions and meteorological conditions are the two main causes of atmospheric pollution, and the contribution of meteorology and emissions to the reduction of PM2.5 concentrations across the country has not yet been comprehensively examined. This study used the Kolmogorov–Zurbenko (KZ) filter and random forest (RF) model to decompose and reconstruct PM2.5 time series in five major urban agglomerations in China, analyzing the impact of meteorological factors on PM2.5 concentrations. From 2015 to 2021, PM2.5 concentrations significantly decreased in all urban agglomerations, with annual averages dropping by approximately 50% in Beijing–Tianjin–Hebei (BTH), Yangtze River Delta (YRD), Pearl River Delta (PRD), Central Plain (CP), and Chengdu–Chongqing (CC). This reduction was due to both favorable meteorological conditions and emission reductions. The KZ filter effectively separated the PM2.5 time series, and the RF model achieved high squared correlation coefficient (R2) values between predicted and observed values, ranging from 0.94 to 0.98. Initially, meteorological factors had a positive contribution to PM2.5 reduction, indicating unfavorable conditions, but this gradually turned negative, indicating favorable conditions. By 2021, the rates of meteorological contribution to PM2.5 reduction in BTH, YRD, PRD, CP, and CC changed from 14.3%, 16.9%, 7.2%, 12.2%, and 11.5% to −36.5%, −31.5%, −26.9%, −30.3%, and −23.5%, respectively. Temperature and atmospheric pressure had the most significant effects on PM2.5 concentrations. The significant decline in PM2.5 concentrations in BTH and CP after 2017 indicated that emission control measures were gradually taking effect. This study confirms that effective pollution control measures combined with favorable meteorological conditions jointly contributed to the improvement in air quality. Full article
(This article belongs to the Special Issue Secondary Atmospheric Pollution Formations and Its Precursors)
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<p>The study area.</p>
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<p>The study’s methodological framework.</p>
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<p>Interannual variations in PM<sub>2.5</sub> concentrations in each urban agglomeration from 2015 to 2021.</p>
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<p>Time series of original PM<sub>2.5</sub> concentrations (black) and meteorologically adjusted PM<sub>2.5</sub> concentrations (colored) for each urban agglomeration.</p>
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<p>Long-term trends of observed (black) and meteorologically adjusted (colored) PM<sub>2.5</sub>.</p>
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<p>Normalized importance of meteorological variables influencing PM<sub>2.5</sub> concentrations in each urban agglomeration.</p>
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<p>Interannual variations in the contribution rates of meteorological factors to the decrease in PM<sub>2.5</sub> concentrations in each urban agglomeration from 2015 to 2021.</p>
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<p>Spatial distribution of the contribution rates of meteorological factors to the decrease in PM<sub>2.5</sub> concentrations in different cities within each urban agglomeration from 2015 to 2021.</p>
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<p>Rate of change in the meteorological contribution to PM<sub>2.5</sub> reduction (colored dots) and its spatial distribution with terrain elevation (colored contours, mean elevation) in each urban agglomeration from 2015 to 2021. (<b>a</b>) BTH, (<b>b</b>) YRD, (<b>c</b>) PRD, (<b>d</b>) CP, (<b>e</b>) CC.</p>
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22 pages, 7731 KiB  
Article
Determining the PM10 Pollution Sources near the Copper Smelter in Bor, Serbia
by Renata Kovačević, Bojan Radović, Dragan Manojlović, Tamara Urošević, Tatjana Apostolovski-Trujić, Viša Tasić and Milena Jovašević-Stojanović
Atmosphere 2024, 15(12), 1498; https://doi.org/10.3390/atmos15121498 - 16 Dec 2024
Abstract
The EPA Positive Matrix Factorization (PMF) 5.0 model was applied to determine the sources and characteristics of PM10 collected near the copper smelter in Bor, Serbia, from September 2009 to July 2010. For a better understanding of the industrial sources of PM [...] Read more.
The EPA Positive Matrix Factorization (PMF) 5.0 model was applied to determine the sources and characteristics of PM10 collected near the copper smelter in Bor, Serbia, from September 2009 to July 2010. For a better understanding of the industrial sources of PM10 pollution, the dataset was divided into four observation periods: heating season (HS), non-heating season (NHS), copper smelter in work (SW), and copper smelter out of work (SOW). The daily limit for the PM10 fraction of 50 μg/m3 was exceeded on one-sixth of days in the NHS, about half the days in the HS, and about one-third of days during the SOW and SW period. The nine different sources of PM10 were identified: fuel combustion, industrial dust, dust from tailings, storage and preparation of raw materials, secondary nitrate, Cu smelter, traffic, cadmium, and plant for the production of precious metals. The contribution of factors related to the activities in the copper smelter complex to the total mass of PM10 was 83.1%. When the copper smelter was out of work the contribution of all the factors related to PM10 pollution from the copper smelter to the total mass of the PM10 was 2.3-fold lower, 35.8%, compared with the period when the copper smelter was in work. This study is the first attempt to use PMF receptor modeling to determine the air pollution sources and their contribution to ambient air pollution in the city of Bor, Serbia. Full article
(This article belongs to the Special Issue Atmospheric Particulate Matter: Origin, Sources, and Composition)
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<p>Location of the sampling site.</p>
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<p>Box plots of PM<sub>10</sub> concentrations for various observation periods: HS (heating season), NHS (non-heating season), SW (copper smelter in work), and SOW (copper smelter out of work).</p>
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<p>Bootstrap box plot factor profiles during the non-heating season.</p>
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<p>Factor contributions during the non-heating season (F<sub>peak</sub> = −0.5).</p>
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<p>Factor fingerprints during the non-heating season (F<sub>peak</sub> = −0.5).</p>
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<p>Bootstrap box plot factor profiles during the heating season.</p>
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<p>Factor contributions during the heating season (F<sub>peak</sub>= −0.1).</p>
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<p>Factor fingerprints during the heating season (F<sub>peak</sub> = −0.1).</p>
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<p>Bootstrap box plot factor profiles in the SOW period.</p>
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<p>Factor contributions during the SOW period (F<sub>peak</sub> = −0.4).</p>
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<p>Factor fingerprints during the SOW period (F<sub>peak</sub> = −0.4).</p>
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<p>Bootstrap box plot factor profiles during the period when the copper smelter works.</p>
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<p>Factor contributions during the period when the smelter works (F<sub>peak</sub>= −0.2).</p>
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<p>Factor fingerprints during the period when the smelter works (F<sub>peak</sub>= −0.2).</p>
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17 pages, 2485 KiB  
Article
Impact of Dust Events on UV Index and Vitamin D Synthesis in Bahrain and Its Correlation with Population Serum 25-Hydroxyvitamin D Levels
by Fatima Jahromi, Maryam Al Mannai, Abdulla Alabed, Saud Alkhlofi, Suha Hejres, Dalal Alromaihi, Prashant Kumar and Afnan Freije
Atmosphere 2024, 15(12), 1497; https://doi.org/10.3390/atmos15121497 - 16 Dec 2024
Viewed by 49
Abstract
Vitamin D plays an important role in maintaining human health. Its deficiency has been associated with an increased risk of several chronic diseases. Sun exposure, particularly UV-B radiation, accounts for greater than 90% of vitamin D production in humans. The aim of this [...] Read more.
Vitamin D plays an important role in maintaining human health. Its deficiency has been associated with an increased risk of several chronic diseases. Sun exposure, particularly UV-B radiation, accounts for greater than 90% of vitamin D production in humans. The aim of this study was to examine the relationship between dust and UV index and its effect on vitamin D concentrations. Data on the UV index and the number of dusty days measured at ≤1000 m, ≤3000 m, and ≤5000 m altitudes in the period January 2017 to June 2022 were collected. Dust particles (PM2.5 and PM10) and vitamin D values were also gathered. No correlation was observed between UV index and PM2.5 (r = −0.013, p = 0.947) and between UV index and PM10 (r = 0.251, p = 0.165) due to numerous factors, such as unavailable data on UV-B and particle concentrations at a maximum of 1000 m rather than 20 to 30 km. A positive correlation was observed between the number of dusty days at all altitudes and PM10 (p < 0.001), whereas no correlation was found between the number of dusty days at all altitudes and PM2.5. A positive correlation was found between vitamin D-deficient patients and PM2.5 (r = 0.529, p = 0.005) and between vitamin D-deficient patients and PM10 (r = 0.399, p = 0.024). The PM 2.5 and PM10 concentrations exceeded both the WHO guidelines and the Environmental Protection Agency’s recommended levels during most months of the study period. The average range of the PM2.5/PM10 ratio was low (0.24–0.35), indicating dust pollution. The results indicate a strong relationship between PM10 dust particles and the number of vitamin D-deficient patients, indicating high levels of dust air pollution, which might have an influence on the high levels of vitamin D deficiency in Bahrain. This study hypothesized that dust events may reduce UV-B levels, leading to vitamin D deficiency (VDD). However, the results of the study supported this hypothesis only partially due to several limitations, including the unavailability of data on UV-B, dusty days, and dust particles (PM2.5 and PM10) at higher altitudes (20–30 Km). Full article
(This article belongs to the Topic Impacts of Air Quality on Environment and Human Health)
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<p>(<b>a</b>) Location of Bahrain within the Arabian Gulf, highlighted by the red triangle, with (<b>b</b>) showing a zoomed-in view [<a href="#B40-atmosphere-15-01497" class="html-bibr">40</a>].</p>
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<p>Summary of the number of dusty days and non-dusty days from January 2017 to June 2022.</p>
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<p>Summary of the number of vitamin D tests and vitamin D-deficient patients from January 2017 to June 2022.</p>
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<p>Residual plots versus number of vitamin D-deficient patients per month using linear regression.</p>
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24 pages, 10007 KiB  
Article
Levels, Sources and Risk Assessment of Carbonaceous and Organic Species Associated with PM2.5 in Two Small Cities of Morelos, Mexico
by Brenda L. Valle-Hernández, José de Jesús Figueroa-Lara, Miguel Torres-Rodríguez, Noé Ginéz-Hernández, Tamara Álvarez-Lupercio and Violeta Mugica-Álvarez
Atmosphere 2024, 15(12), 1496; https://doi.org/10.3390/atmos15121496 - 15 Dec 2024
Viewed by 624
Abstract
A study of carbonaceous species, polycyclic aromatic hydrocarbons (PAHs), and nitro-PAHs associated with PM2.5 was conducted to assess their carcinogenic potential and associated health risks in the two main cities of the State of Morelos: Cuernavaca and Cuautla. The annual median concentrations [...] Read more.
A study of carbonaceous species, polycyclic aromatic hydrocarbons (PAHs), and nitro-PAHs associated with PM2.5 was conducted to assess their carcinogenic potential and associated health risks in the two main cities of the State of Morelos: Cuernavaca and Cuautla. The annual median concentrations in Cuernavaca of organic carbon (OC) and elemental carbon (EC) were 6.2 µg m−3 and 0.6 µg m−3, respectively, whereas in Cuautla, OC concentrations averaged 4.8 µg m−3 and EC 0.6 µg m−3. OC/EC ratios, total carbonaceous aerosols (TCA), primary (POC) and secondary organic carbon (SOC), as well as elemental carbon reactive (ECR) were estimated, also showing prevalence of primary emissions such as biomass burning. The seventeen PAHs recommended by the EPA and twelve nitro-PAHs were measured using gas chromatography–mass spectrometry. The annual median sum of PAHs was 9.7 ng m−3 in Cuernavaca and 11.2 ng m−3 in Cuautla, where carcinogenic high-molecular-weight compounds were the most dominant; the annual median sums of nitro-PAHs were 287 pg m−3 and 432 pg m−3, respectively. Diagnostic ratios were applied to identify potential sources of PAH emissions, suggesting that fuel combustion is the major contributor in both sites, followed by coal biomass burning and agricultural activities. The annual carcinogenic potential as benzo(a)pyrene equivalent was 2.2 ng m−3 for both sites. The lifetime excess cancer risk from PAH inhalation was estimated to range from 1.8 × 10−4 to 2 × 10−4 in Cuernavaca and from 1.5 × 10−4 to 2.2 × 10−4 in Cuautla, similar to values observed in other urban regions globally. Full article
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<p>Sampling sites (Cuernavaca and Cuautla) in the State of Morelos, Mexico.</p>
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<p>Time series graph of OC and EC concentrations from the two sampling sites.</p>
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<p>Medians of OC and EC concentrations by season and site. Box: 25–75%; Whisker: 10–90%.</p>
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<p>Concentration charts of OC, EC, and PAHs for Cuernavaca (CUE).</p>
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<p>Concentration charts of OC, EC, and PAHs for CUA.</p>
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<p>Relationships of organic carbon (OC) and elemental carbon (EC) in PM<sub>2.5</sub> correlations for (<b>a</b>) Cuernavaca (CUE) and (<b>b</b>) Cuautla (CUA).</p>
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<p>OC/EC ratio in Cuernavaca (CUE) and Cuautla (CUA) by season.</p>
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<p>Median Primary Organic Concentration (POC) and Secondary Organic concentration (SOC), and % SOC/OC by season and site.</p>
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<p>Median concentration of PAHs associated with PM<sub>2.5</sub> in Cuernavaca by season.</p>
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<p>Median concentration of PAHs associated with PM<sub>2.5</sub> in Cuautla by season.</p>
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<p>Median concentration of PAHsum and PAHcarcinogenic; Box: 25–75%; Whisker: 10–90%.</p>
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<p>Seasonal median concentration of nitro-PAHs in PM<sub>2.5</sub> in Cuernavaca (<b>a</b>) and Cuautla (<b>b</b>).</p>
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<p>Flt vs. 2-NFlt in CUE. (<b>a</b>) Warm-dry and (<b>b</b>) Rainy seasons.</p>
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<p>Median concentrations (10 and 90 percentiles) of nitro-PAHs in PM<sub>2.5</sub> in CUE and CUA, during R, WD, and CD seasons. Median; Box: 25–75%; Whisker: 10–90%.</p>
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<p><b>Seasonal</b> BaPeq concentrations in Cuernavaca and Cuautla.</p>
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12 pages, 2228 KiB  
Article
The Radon Exhalation Rate and Dose Assessment of Granite Used as a Building Material in Serbia
by Fathya Shabek, Božidar Obradović, Igor Čeliković, Mirjana Đurašević, Aleksandra Samolov, Predrag Kolarž and Aco Janićijević
Atmosphere 2024, 15(12), 1495; https://doi.org/10.3390/atmos15121495 - 15 Dec 2024
Viewed by 420
Abstract
The application of energy-saving policies in buildings could lead to a decrease in the air exchange rate in dwellings, which could consequently lead to an increase in indoor radon concentration and, therefore, to an increase in resident exposure to ionizing radiation. The aim [...] Read more.
The application of energy-saving policies in buildings could lead to a decrease in the air exchange rate in dwellings, which could consequently lead to an increase in indoor radon concentration and, therefore, to an increase in resident exposure to ionizing radiation. The aim of the research presented in this paper is to investigate radiological exposure to residents due to the usage of different granites commonly used in Serbia as a building material. From the total of 10 analysed granite samples, a wide range of radon and thoron exhalation rates were found: from <161 μBq m−2 s−1 to 5220 ± 200 μBq m−2 s−1 and from <7 mBq m−2 s−1 to 5140 ± 320 mBq m−2 s−1, respectively. Assuming a low air exchange rate of 0.2 h−1, the contribution of the measured granite material to the indoor radon concentration could go up to 150 Bq m−3. The estimated annual effective doses due to exposure to radon and thoron exhalation from the granite samples were (0.05–3.79) mSv and (<0.01–1.74) mSv, respectively. The specific activity of radionuclides ranged from 6.6 ± 0.5 Bq kg−1 to 131.8 ± 9.4 Bq kg−1 for 226Ra, from 0.5 ± 0.1 Bq kg−1 to 120.8 ± 6.5 Bq kg−1 for 232Th, and from 0.22 ± 0.01 Bq kg−1 to 1321 ± 86 Bq kg−1 for 40K. The obtained external hazard index ranged from 0.03 to 1.48, with three samples above or very close to the accepted safety limit of 1. In particular, dwellings with a low air exchange rate (causing elevated radon) could lead to an elevated risk of radiation exposure. Full article
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<p>Schematic drawing of radon exhalation rate measurement.</p>
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<p>The build-up of radon exhaling from Sample 1 in a 30 L accumulation chamber. Experimental data are fitted on a theoretical curve given by Equation (1). From the fit, values of <span class="html-italic">E<sub>S</sub></span>, <span class="html-italic">C</span><sub>0</sub>, and <span class="html-italic">λ<sub>eff</sub></span> are extracted.</p>
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<p>Radon and thoron surface exhalation rates from 10 different granite samples obtained using the closed-chamber accumulation method.</p>
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<p>Specific activities of <sup>226</sup>Ra, <sup>232</sup>Tn, and <sup>40</sup>K of 10 selected granite samples.</p>
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<p>The annual effective doses due to the inhalation of radon (<span class="html-italic">λ<sub>v</sub></span> = 0.2 h<sup>−1</sup>) and thoron (EECT), as well as due to the exposure to external radiation.</p>
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<p>External hazard index.</p>
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12 pages, 3041 KiB  
Article
High-Spatial Resolution Maps of PM2.5 Using Mobile Sensors on Buses: A Case Study of Teltow City, Germany, in the Suburb of Berlin, 2023
by Jean-Baptiste Renard, Günter Becker, Marc Nodorft, Ehsan Tavakoli, Leroy Thiele, Eric Poincelet, Markus Scholz and Jérémy Surcin
Atmosphere 2024, 15(12), 1494; https://doi.org/10.3390/atmos15121494 - 15 Dec 2024
Viewed by 299
Abstract
Air quality monitoring networks regulated by law provide accurate but sparse measurements of PM2.5 mass concentrations. High-spatial resolution maps of the PM2.5 mass concentration values are necessary to better estimate the citizen exposure to outdoor air pollution and the sanitary consequences. To address [...] Read more.
Air quality monitoring networks regulated by law provide accurate but sparse measurements of PM2.5 mass concentrations. High-spatial resolution maps of the PM2.5 mass concentration values are necessary to better estimate the citizen exposure to outdoor air pollution and the sanitary consequences. To address this, a field campaign was conducted in Teltow, a midsize city southwest of Berlin, Germany, for the 2021–2023 period. A network of optical sensors deployed by Pollutrack included fixed monitoring stations as well as mobile sensors mounted on the roofs of buses and cars. This setup provides PM2.5 pollution maps with a spatial resolution down to 100 m on the main roads. The reliability of Pollutrack measurements was first established with comparison to measurements from the German Environment Agency (UBA) and modelling calculations based on high-resolution weather forecasts. Using these validated data, maps were generated for 2023, highlighting the mean PM2.5 mass concentrations and the number of days per year above the 15 µg.m−3 value (the daily maximum recommended by the World Health Organization (WHO) in 2021). The findings indicate that PM2.5 levels in Teltow are generally in the good-to-moderate range. The higher values (hot spots) are detected mainly along the highways and motorways, where traffic speeds are higher compared to inner-city roads. Also, the PM2.5 mass concentrations are higher on the street than on the sidewalks. The results were further compared to those in the city of Paris, France, obtained using the same methodology. The observed parallels between the two datasets underscore the strong correlation between traffic density and PM2.5 concentrations. Finally, the study discusses the advantages of integrating such high-resolution sensor networks with modelling approaches to enhance the understanding of localized PM2.5 variability and to better evaluate public exposure to air pollution. Full article
(This article belongs to the Special Issue Cutting-Edge Developments in Air Quality and Health)
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<p>A map of the south suburb of Berlin, including Teltow; the red dot represents the PM2.5 reference station and the purple dot represents Pollutrack fixed stations (north is up).</p>
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<p>Pollutrack sensors (inside the red circle) on the roof of a bus (<b>left</b>) and of a car (<b>right</b>).</p>
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<p>The time evolution of the PM2.5 concentrations for the UBA reference station, the Pollutrack fixed stations, and the modelling calculation.</p>
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<p>Histograms of the difference for the cross-comparison sessions of measurements (a sliding smoothing over 3 consecutive points is applied for the differences involving the modelling data due to a lower number of datapoints).</p>
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<p>Locations of the measurements; black dots: sparse measurements; red dots: regular measurements.</p>
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<p>Mean PM2.5 mass concentrations from mobile sensors (thick square) and fixed sensors (thick crosses) superimposed on main roads in pale orange and secondary roads in pale grey.</p>
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<p>The installation of the fixed sensors.</p>
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<p>The mean number of days with PM2.5 mass concentrations above 15 µg.m<sup>−3</sup> from the mobile sensors (thick square) superimposed on main roads in pale orange and secondary roads in pale grey.</p>
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11 pages, 4025 KiB  
Article
Experimental Research on Permeability and Effective Radon Reduction of Chemical Solidification of Uranium Tailings
by Jindong Wang and Shuai Zhang
Atmosphere 2024, 15(12), 1493; https://doi.org/10.3390/atmos15121493 - 14 Dec 2024
Viewed by 425
Abstract
To be able to study the permeability coefficient and radon reduction effect of three materials before and after the solidification of uranium tailings. Firstly, uranium tailings, blast furnace slag, lime, fly ash and cement were selected as raw materials for the experiment. Three [...] Read more.
To be able to study the permeability coefficient and radon reduction effect of three materials before and after the solidification of uranium tailings. Firstly, uranium tailings, blast furnace slag, lime, fly ash and cement were selected as raw materials for the experiment. Three solidified materials were mixed with 7.5%, 10% and 12.5% of equal proportions of cement. The curing samples of nine kinds of solidified bodies were prepared after curing. Subsequently, the permeability coefficient was determined through the utilization of X-ray diffraction (XRD) and scanning electron microscopy (SEM). And cumulative radon concentrations in uranium tailings and samples were measured by RAD7. Thus, the radon exhalation rate of the original sample and the sample were determined. The experimental results show that the permeability coefficient of nine samples decreased with the quadratic function with the increase in the amount of curing agent. Microscopic scanning results show that there is a positive correlation among the radon exhalation rate, permeability coefficient and cementation degree. The best material for solidifying uranium tailings and radon insulation was blast furnace slag, followed by fly ash. Full article
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<p>XRD patterns of fly ash samples.</p>
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<p>SEM images of uranium tailing sample.</p>
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<p>Scanning electron microscopy results of uranium tailings and samples mixed with different curing agents.</p>
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<p>The permeability coefficient curve of each sample.</p>
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<p>Uranium tailings and single-sided radon exhalation rate curve of each sample.</p>
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<p>Relationship between permeability coefficient and radon exhalation rate of each sample.</p>
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22 pages, 1684 KiB  
Article
Evaluating Ionospheric Total Electron Content (TEC) Variations as Precursors to Seismic Activity: Insights from the 2024 Noto Peninsula and Nichinan Earthquakes of Japan
by Karan Nayak, Rosendo Romero-Andrade, Gopal Sharma, Charbeth López-Urías, Manuel Edwiges Trejo-Soto and Ana Isela Vidal-Vega
Atmosphere 2024, 15(12), 1492; https://doi.org/10.3390/atmos15121492 - 14 Dec 2024
Viewed by 217
Abstract
This study provides a comprehensive investigation into ionospheric perturbations associated with the Mw 7.5 earthquake on the Noto Peninsula in January 2024, utilizing data from the International GNSS Service (IGS) network. Focusing on Total Electron Content (TEC), the analysis incorporates spatial mapping and [...] Read more.
This study provides a comprehensive investigation into ionospheric perturbations associated with the Mw 7.5 earthquake on the Noto Peninsula in January 2024, utilizing data from the International GNSS Service (IGS) network. Focusing on Total Electron Content (TEC), the analysis incorporates spatial mapping and temporal pattern assessments over a 30-day period before the earthquake. The time series for TEC at the closest station to the epicenter, USUD, reveals a localized decline, with a significant negative anomaly exceeding 5 TECU observed 22 and 23 days before the earthquake, highlighting the potential of TEC variations as seismic precursors. Similar patterns were observed at a nearby station, MIZU, strengthening the case for a seismogenic origin. Positive anomalies were linked to intense space weather episodes, while the most notable negative anomalies occurred under geomagnetically calm conditions, further supporting their seismic association. Using Kriging interpolation, the anomaly zone was shown to closely align with the earthquake’s epicenter. To assess the consistency of TEC anomalies in different seismic events, the study also examines the Mw 7.1 Nichinan earthquake in August 2024. The results reveal a prominent negative anomaly, reinforcing the reliability of TEC depletions in seismic precursor detection. Additionally, spatial correlation analysis of Pearson correlation across both events demonstrates that TEC coherence diminishes with increasing distance, with pronounced correlation decay beyond 1000–1600 km. This spatial decay, consistent with Dobrovolsky’s earthquake preparation area, strengthens the association between TEC anomalies and seismic activity. This research highlights the complex relationship between ionospheric anomalies and seismic events, underscoring the value of TEC analysis as tool for earthquake precursor detection. The findings significantly enhance our understanding of ionospheric dynamics related to seismic events, advocating for a comprehensive, multi-station approach in future earthquake prediction efforts. Full article
30 pages, 28793 KiB  
Article
An Investigation of the SOCOLv4 Model’s Suitability for Predicting the Future Evolution of the Total Column Ozone
by Georgii Nerobelov, Yurii Timofeyev, Alexander Polyakov, Yana Virolainen, Eugene Rozanov and Vladimir Zubov
Atmosphere 2024, 15(12), 1491; https://doi.org/10.3390/atmos15121491 - 14 Dec 2024
Viewed by 226
Abstract
The anthropogenic impact on the ozone layer is expressed in anomalies in the total ozone content (TOC) on a global scale, with periodic enhancements observed in high-latitude areas. In addition, there are significant variations in TOC time trends at different latitudes and seasons. [...] Read more.
The anthropogenic impact on the ozone layer is expressed in anomalies in the total ozone content (TOC) on a global scale, with periodic enhancements observed in high-latitude areas. In addition, there are significant variations in TOC time trends at different latitudes and seasons. The reliability of the TOC future trends projections using climate chemistry models must be constantly monitored and improved, exploiting comparisons against available measurements. In this study, the ability of the Earth’s system model SOCOLv4.0 to predict TOC is evaluated by using more than 40 years of satellite measurements and meteorological reanalysis data. In general, the model overpredicts TOC in the Northern Hemisphere (by up to 16 DU) and significantly underpredicts it in the South Pole region (by up to 28 DU). The worst agreement was found in both polar regions, while the best was in the tropics (the mean difference constitutes 4.2 DU). The correlation between monthly means is in the range of 0.75–0.92. The SOCOLv4 model significantly overestimates air temperature above 1 hPa relative to MERRA2 and ERA5 reanalysis (by 10–20 K), particularly during polar nights, which may be one of the reasons for the inaccuracies in the simulation of polar ozone anomalies by the model. It is proposed that the SOCOLv4 model can be used for future projections of TOC under the changing scenarios of human activities. Full article
(This article belongs to the Special Issue Measurement and Variability of Atmospheric Ozone)
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<p>Global distribution of mean differences or MD (<b>a</b>), SDD (<b>b</b>), and correlation coefficients (<b>c</b>) between TOC by SOCOLv4 modeling and satellite observations (CAMS MSR for 1980–2022—<b>left</b>, IKFS-2 for 2015–2022—<b>middle</b>, IASI for 2008–2023—<b>right</b>).</p>
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<p>Seasonal global distribution of mean differences or MD (<b>left</b>), SDD (<b>center</b>), and correlation coefficients (<b>right</b>) between TOC by SOCOLv4 modeling and combined satellite observations in CAMS MSR dataset in winter (JJA, (<b>a</b>)), spring (MAM, (<b>b</b>)), summer (JJA, (<b>c</b>)) and autumn (SON, (<b>d</b>)) for 1980–2022.</p>
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<p>Monthly mean TOC averaged in zones 70–90° N (<b>a</b>) and 70–90° S (<b>b</b>) by SOCOLv4 modeling (ensemble member mean) and CAMS MSR dataset for 1980–2022 and their differences (SOCOLv4 minus obs.).</p>
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<p>Monthly mean TOC averaged in zones 70–90° N (<b>a</b>) and 70–90° S (<b>b</b>) by SOCOLv4 modeling (ensemble member mean) and satellite observations (IASI—2008–2023, IKFS-2—2015–2022) and their differences (SOCOLv4 minus obs.).</p>
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<p>Monthly and globally averaged mean TOCs from SOCOLv4 modeling (ensemble member mean) and CAMS MSR and their differences (SOCOLv4 minus CAMS MSR).</p>
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<p>Deseasonolized monthly and globally averaged mean TOCs from SOCOLv4 modeling (ensemble member mean) and CAMS MSR for 1980–1992 (<b>a</b>) and 1993–2022 (<b>b</b>) and their regression lines.</p>
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<p>Zonal distribution of mean difference ((<b>a</b>), MD), its SDD (<b>b</b>), and correlation (CC, (<b>c</b>)) between air temperature from SOCOLv4 and reanalysis (ERA5 on the left and MERRA2 on the right) data for 1980–2023; dots indicate statistically insignificant differences according to <span class="html-italic">t</span>-test (0.95 confidence level).</p>
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<p>Monthly mean air temperature averaged in zone 60–90° N at 100 hPa (<b>a</b>) and 1 hPa (<b>b</b>) by SOCOLv4 modeling (ensemble member mean) and reanalysis data (ERA5 and MERRA2) for DJF 1980–2023 and their differences (SOCOLv4 minus reanalysis).</p>
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<p>Monthly mean air temperature averaged in zone 60–90° N at 100 hPa (<b>a</b>) and 1 hPa (<b>b</b>) by SOCOLv4 modeling (ensemble member mean) and reanalysis data (ERA5 and MERRA2) for DJF 1980–2023 and their differences (SOCOLv4 minus reanalysis).</p>
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<p>Zonal distribution of R<sup>2</sup> between air temperature from SOCOLv4 (<b>a</b>) and reanalysis data (ERA5—(<b>b</b>), MERRA2—(<b>c</b>)) and MLR model data for 1980–2022; black dots depict zones where MLR model is statistically significant at a 0.95 confidence level.</p>
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<p>Zonal distribution of decadal trend of deseasonalized air temperature from SOCOLv4 (<b>a</b>) and reanalysis data (ERA5—(<b>b</b>), MERRA2—(<b>c</b>)) for 1980–2022; dashed line depicts the area of R<sup>2</sup> ≥ 0.5 (between deseasonalized air temperature and linear regression).</p>
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<p>Time series of MLR predictors ((<b>a</b>)—CHC-11 content, (<b>b</b>)—ENSO parameter, (<b>c</b>)—QBO parameter, (<b>d</b>)—solar radiation in radio range, (<b>e</b>)—AOD).</p>
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<p>Zonal distribution of mean differences or MD, SDD of MD, and correlation coefficients between TOC from SOCOLv4 modelling and satellite observations (CAMS MSR for 1980–2022—(<b>a</b>), IKFS-2 for 2015–2022—(<b>b</b>), IASI for 2008–2023—(<b>c</b>)).</p>
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<p>Zonal distribution of mean differences or MD, SDD of MD, and correlation coefficients between TOC from SOCOLv4 modelling and satellite observations (CAMS MSR for 1980–2022—(<b>a</b>), IKFS-2 for 2015–2022—(<b>b</b>), IASI for 2008–2023—(<b>c</b>)).</p>
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<p>Zonal distribution of mean difference (MD) between air temperature from SOCOLv4 and reanalysis data (ERA5 on the left, MERRA2 on the right) for winter (<b>a</b>), spring (<b>b</b>), summer (<b>c</b>), and autumn (<b>d</b>) 1980–2023; dots indicate statistical insignificant differences according to <span class="html-italic">t</span>-test (0.95 confidence level).</p>
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<p>Zonal distribution of mean difference (MD) between air temperature from SOCOLv4 and reanalysis data (ERA5 on the left, MERRA2 on the right) for winter (<b>a</b>), spring (<b>b</b>), summer (<b>c</b>), and autumn (<b>d</b>) 1980–2023; dots indicate statistical insignificant differences according to <span class="html-italic">t</span>-test (0.95 confidence level).</p>
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<p>Zonal distribution of the SDD between air temperature from SOCOLv4 and reanalysis data (ERA5 on the left, MERRA2 on the right) for winter(<b>a</b>), spring (<b>b</b>), summer (<b>c</b>), and autumn (<b>d</b>) 1980–2023; dots indicate statistical insignificant differences according to <span class="html-italic">t</span>-test (0.95 confidence level).</p>
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<p>Zonal distribution of the SDD between air temperature from SOCOLv4 and reanalysis data (ERA5 on the left, MERRA2 on the right) for winter(<b>a</b>), spring (<b>b</b>), summer (<b>c</b>), and autumn (<b>d</b>) 1980–2023; dots indicate statistical insignificant differences according to <span class="html-italic">t</span>-test (0.95 confidence level).</p>
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<p>Zonal distribution of the correlation coeffitients between air temperature from SOCOLv4 and reanalysis data (ERA5 on the left, MERRA2 on the right) for winter (<b>a</b>), spring (<b>b</b>), summer (<b>c</b>), and autumn (<b>d</b>) 1980–2023; dots indicate statistical insignificant differences according to <span class="html-italic">t</span>-test (0.95 confidence level).</p>
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<p>Zonal distribution of the correlation coeffitients between air temperature from SOCOLv4 and reanalysis data (ERA5 on the left, MERRA2 on the right) for winter (<b>a</b>), spring (<b>b</b>), summer (<b>c</b>), and autumn (<b>d</b>) 1980–2023; dots indicate statistical insignificant differences according to <span class="html-italic">t</span>-test (0.95 confidence level).</p>
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<p>Monthly mean air temperature averaged in zone 60–90° N at 100 hPa (<b>a</b>) and 1 hPa (<b>b</b>) by SOCOLv4 modelling (ensemble member mean) and reanalysis data (ERA5 and MERRA2) for 1980–2023 and their differences (SOCOLv4 minus reanalysis).</p>
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<p>Monthly mean air temperature averaged in zone 60–90° N at 100 hPa (<b>a</b>) and 1 hPa (<b>b</b>) by SOCOLv4 modelling (ensemble member mean) and reanalysis data (ERA5 and MERRA2) for 1980–2023 and their differences (SOCOLv4 minus reanalysis).</p>
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25 pages, 6134 KiB  
Article
The Impact of Ecological Governance Projects on Regional Ecological Carrying Capacity Under Climate Change
by Shaobo Liu
Atmosphere 2024, 15(12), 1490; https://doi.org/10.3390/atmos15121490 - 13 Dec 2024
Viewed by 254
Abstract
Ecological governance projects have great potential benefits, but there is a lack of quantitative evaluation of their impacts in terms of enhancing regional ecological carrying capacity under climate change. To quantitatively evaluate the impact of ecological governance projects on regional ecological carrying capacity, [...] Read more.
Ecological governance projects have great potential benefits, but there is a lack of quantitative evaluation of their impacts in terms of enhancing regional ecological carrying capacity under climate change. To quantitatively evaluate the impact of ecological governance projects on regional ecological carrying capacity, a quantitative evaluation model was developed by coupling the classical ecological footprint and ecological service value theory. This model was validated using the water source treatment project (hereinafter referred to as the “DZ” project) of the Middle Route of China’s South to North Water Diversion Project, which is the world’s largest water diversion project, as an example. The results showed the following: (1) During the implementation of the “DZ” project, the per capita ecological carrying capacity of the reservoir area experienced a wave-like growth trend, with an increase of 0.103615 hm2 and a yield increase rate of 20.00%. The “DZ” project has outstanding ecological benefits, valued at approximately USD 125.272266 million. (2) The “DZ” project has contributed to the improvement of the ecological carrying capacity in the Henan area of the Danjiang Reservoir by about 10.14%, demonstrating that such projects have a considerable impact on efforts to improve regional ecological carrying capacity under climate change. Full article
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<p>The specific geographical location and the topography of the Henan Reservoir area of the Danjiangkou Reservoir.</p>
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<p>The changes in rainfall of the Henan Reservoir area of the Danjiangkou Reservoir.</p>
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<p>Application process of ecological footprint model.</p>
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<p>Schematic diagram of the value of conserving water sources.</p>
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<p>Schematic diagram of the value of flood control.</p>
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<p>Schematic diagram of the value of purifying water quality.</p>
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<p>Schematic diagram of the value of storing nutritional components.</p>
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<p>Schematic diagram of the value of protecting land resources.</p>
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<p>Schematic diagram of the value of reducing sediment accumulation in reservoirs.</p>
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<p>Schematic diagram of the value of carbon sequestration and oxygen supply.</p>
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<p>Schematic diagram of the value of purifying the air.</p>
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<p>Per capita ecological footprint changes in the Danjiangkou Reservoir area of Henan Province (2006–2016).</p>
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<p>Ecological indicators of Danjiangkou Reservoir area in Henan Province from 2006 to 2016.</p>
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<p>Ecological service value of the “DZ” project.</p>
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19 pages, 20601 KiB  
Article
The Influence of Climate Change and Socioeconomic Transformations on Land Use and NDVI in Ordos, China
by Yin Cao, Zhigang Ye and Yuhai Bao
Atmosphere 2024, 15(12), 1489; https://doi.org/10.3390/atmos15121489 - 13 Dec 2024
Viewed by 332
Abstract
Land use change is related to a series of core issues of global environmental change, such as environmental quality improvement, sustainable utilization of resources, energy reuse and climate change. In this study, Google Earth Engine (GEE), a remote sensing natural environment monitoring and [...] Read more.
Land use change is related to a series of core issues of global environmental change, such as environmental quality improvement, sustainable utilization of resources, energy reuse and climate change. In this study, Google Earth Engine (GEE), a remote sensing natural environment monitoring and analysis platform, was used to realize the combination of Landsat TM/OLI data images with spectral features and topographic features, and the random forest machine learning classification method was used to supervise and classify the low-cloud composite image data of Ordos City. The results show that: (1) GEE has a powerful computing function, which can realize efficient and high-precision in-depth analysis of long-term multi-temporal remote sensing images and monitoring of land use change, and the accuracy of acquisition can reach 87%. Compared with other data sets in the same period, the overall and local classification results are more distinct than ESRI (Environmental Systems Research Institute) and GlobeLand 30 data products. Slightly lower than the Institute of Aerospace Information Innovation of the Chinese Academy of Sciences to obtain global 30 m of land cover fine classification products. (2) The overall accuracy of the land cover data of Ordos City from 2003 to 2023 is between 79–87%, and the Kappa coefficient is between 0.79–0.84. (3) Climate, terrain, population and other interactive factors combined with socio-economic population data and national and local policies are the main factors affecting land use change between 2003 and 2023. Full article
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<p>Ordos city bitmap.</p>
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<p>Technique flow chart.</p>
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<p>Comparison of the importance of different features.</p>
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<p>Area changes for each land use/land cover type: (<b>a</b>) Cultivated Land; (<b>b</b>) Forest Land; (<b>c</b>) Grassland; (<b>d</b>) Water Body; (<b>e</b>) Built-up Land; (<b>f</b>) Unused Land.</p>
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<p>Land Use Change Map of Ordos City: (<b>a</b>) 2003; (<b>b</b>) 2008; (<b>c</b>) 2013; (<b>d</b>) 2018; (<b>e</b>) 2023.</p>
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<p>Ordos City time series (2003–2023): (<b>a</b>) Rainfall; (<b>b</b>) LST.</p>
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<p>Economic Development Indicators of Ordos City from 2003 to 2022: (<b>a</b>) gross regional domestic product; (<b>b</b>) Total output of three industries.</p>
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<p>Livelihood Development Indicators of Ordos City from 2003 to 2022: (<b>a</b>) GDP per capita; (<b>b</b>) Per capita income.</p>
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<p>Urbanization Development Indicators from 2003 to 2022: (<b>a</b>) urbanization rate; (<b>b</b>) Year-end population.</p>
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<p>(<b>a</b>) The trend of NDVI changes in Ordos from 2003 to 2023; (<b>b</b>) The spatial distribution of NDVI change trends in Ordos from 2003 to 2023.</p>
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<p>Significant NDVI trend changes in Ordos from 2003 to 2023.</p>
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14 pages, 3274 KiB  
Article
Reconstructed Phase Space of Tropical Cyclone Activity in the North Atlantic Basin for Determining the Predictability of the System
by Sarah M. Weaver, Christopher A. Steward, Jason J. Senter, Sarah S. Balkissoon and Anthony R. Lupo
Atmosphere 2024, 15(12), 1488; https://doi.org/10.3390/atmos15121488 - 12 Dec 2024
Viewed by 457
Abstract
Tropical cyclone prediction is often described as chaotic and unpredictable on time scales that cross into stochastic regimes. Predictions are bounded by the depth of understanding and the limitations of the physical dynamics that govern them. Slight changes in global atmospheric and oceanic [...] Read more.
Tropical cyclone prediction is often described as chaotic and unpredictable on time scales that cross into stochastic regimes. Predictions are bounded by the depth of understanding and the limitations of the physical dynamics that govern them. Slight changes in global atmospheric and oceanic conditions may significantly alter tropical cyclone genesis regions and intensity. The purpose of this paper is to characterize the predictability of seasonal storm characteristics in the North Atlantic basin by utilizing the Largest Lyapunov Exponent and Takens’ Theorem, which is rarely used in weather or climatological analysis. This is conducted for a post-weather satellite era (1960–2022). Based on the accumulated cyclone energy (ACE) time series in the North Atlantic basin, cyclone activity can be described as predictable at certain timescales. Insight and understanding into this coupled non-linear system through an analysis of time delay, embedded dimension, and Lyapunov exponent-reconstructed phase space have provided critical information for the system’s predictability. Full article
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<p>The study region. The Atlantic Region as provided by the National Hurricane Center, 2022 [<a href="#B20-atmosphere-15-01488" class="html-bibr">20</a>].</p>
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<p>A time series graph of yearly <span class="html-italic">ACE</span> (red—× 10<sup>4</sup> kt<sup>2</sup>), the linear regression trend of <span class="html-italic">ACE</span> (blue line), and named storms (blue) from 1851 to 2022. The correlation between <span class="html-italic">ACE</span> and named storms = 0.73, <span class="html-italic">p</span> = 0.01.</p>
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<p>A line graph showing the accumulated cyclone energy ACE (red) in comparison to the year and PDO Index (blue) for the North Atlantic Ocean.</p>
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<p>Time series based on accumulated cyclone energy (red × 10<sup>4</sup> kt<sup>2</sup>) computed via Python for the years 1851–2022. The blue line is the ‘centered’ running mean.</p>
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<p>A graph of the time delay against mutual information for the annual values of <span class="html-italic">ACE</span> (1960–2022) showing the first local minimum. The time delay was determined to be one. The green dased line represents the threshold of e<sup>−1</sup>.</p>
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<p>A graph of <span class="html-italic">E</span>1(<span class="html-italic">d</span>) and <span class="html-italic">E</span>2(<span class="html-italic">d</span>) against dimensions (<span class="html-italic">d</span>) for the <span class="html-italic">ACE</span> (1960 to 2022). The embedding dimension was determined to be six.</p>
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<p>Takens’ reconstructed phase space for accumulated cyclone energy from 1960 to 2022. The abscissa is the unfiltered time series, the ordinate is the time series with a lag of one year, and the applicate is the time series with a lag of two years.</p>
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<p>The maximum Lyapunov exponent of accumulated cyclone energy is 0.084.</p>
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<p>Takens’ reconstructed phase space for SSTs from 1960 to 2019. The abscissa is the unfiltered time series, the ordinate is the time series with a lag of one year, and the applicate is the time series with a lag of two years.</p>
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10 pages, 3126 KiB  
Article
Comparison of the Contrail Drift Parameters Calculated Based on the Radiosonde Observation and ERA5 Reanalysis Data
by Ilia Bryukhanov, Oleg Loktyushin, Evgeny Ni, Ignatii Samokhvalov, Konstantin Pustovalov and Olesia Kuchinskaia
Atmosphere 2024, 15(12), 1487; https://doi.org/10.3390/atmos15121487 (registering DOI) - 12 Dec 2024
Viewed by 269
Abstract
Aircraft contrails exhibit optical properties similar to those of natural high-level clouds (HLCs) and also form persistent cirrus cloudiness. This paper outlines a methodology for detecting and identifying contrails based on the joint analysis of aircraft trajectories (ADS-B monitoring), the vertical profiles of [...] Read more.
Aircraft contrails exhibit optical properties similar to those of natural high-level clouds (HLCs) and also form persistent cirrus cloudiness. This paper outlines a methodology for detecting and identifying contrails based on the joint analysis of aircraft trajectories (ADS-B monitoring), the vertical profiles of meteorological parameters (radiosonde observation (RAOB) and ERA5 reanalysis), and polarization laser sensing data obtained with the matrix polarization lidar. The potential application of ERA5 reanalysis for determining contrail drift parameters (azimuth, speed, distance, duration, and time of the contrail appearance above the lidar) and interpreting atmospheric polarization laser sensing data in terms of the presence of crystalline ice particles and the assessment of the degree of their horizontal orientation is demonstrated. In the examined case (6 February 2023; Boeing 777-F contrail; flight altitude of 10.3 km; HLC altitude range registered with the lidar of 9.5–10.3 km), the difference in the times of appearance of the contrail over the lidar, calculated from RAOB and ERA5 data, did not exceed 10 min. The difference in the wind direction was 12°, with a wind speed difference of 2 m/s, and the drift distance was approximately the same at about 30 km. The demonstrated technique will allow the experimental dataset of contrail optical and microphysical characteristics to be enhanced and empirical relationships between these characteristics and meteorological quantities to be established. Full article
(This article belongs to the Section Atmospheric Techniques, Instruments, and Modeling)
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<p>HAMPL system layout includes the following components: 1—laser source; 2—Glan–Taylor prism; 3—lens collimator; 4—stepper motor unit; 5—polarization control unit; 6—Cassegrain mirror telescope; 7—aperture stop; 8—converging lens; 9—interference filter; 10—Wollaston prism; 11—photomultiplier tubes; 12—electro-optic shutters; 13—computerized equipment for data acquisition and visualization [<a href="#B20-atmosphere-15-01487" class="html-bibr">20</a>].</p>
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<p>Weather stations within a radius of 500 km from Tomsk [<a href="#B20-atmosphere-15-01487" class="html-bibr">20</a>].</p>
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<p>Fragment of the aircraft flight trajectory [<a href="#B22-atmosphere-15-01487" class="html-bibr">22</a>] near the NR TSU HAMPL location.</p>
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<p>Dynamics of the vertical profile of the lidar signal intensity (6 February 2023; 13:10:49–13:27:31).</p>
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<p>Vertical profile of the lidar signal intensity summed up during a series of measurements on 6 February 2023; 13:10:49–13:27:31).</p>
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19 pages, 12447 KiB  
Article
Characteristics of Strong Cooling Events in Winter of Northeast China and Their Association with 10–20 d Atmosphere Low-Frequency Oscillation
by Qianhao Wang and Liping Li
Atmosphere 2024, 15(12), 1486; https://doi.org/10.3390/atmos15121486 (registering DOI) - 12 Dec 2024
Viewed by 314
Abstract
In the past 42 years from 1980 to 2021, 103 regional strong cooling events (RSCEs) occurred in winter in Northeast China, and the frequency has increased significantly in the past 10 years, averaging 2.45 per year. The longest (shortest) duration is 10 (2) [...] Read more.
In the past 42 years from 1980 to 2021, 103 regional strong cooling events (RSCEs) occurred in winter in Northeast China, and the frequency has increased significantly in the past 10 years, averaging 2.45 per year. The longest (shortest) duration is 10 (2) days. The minimum temperature series in 60 events exists in 10–20 d of significant low-frequency (LF) periods. The key LF circulation systems affecting RSCEs include the Lake Balkhash–Baikal ridge, the East Asian trough (EAT), the robust Siberian high (SH) and the weaker (stronger) East Asian temperate (subtropical) jet, with the related anomaly centers moving from northwest to southeast and developing into a nearly north–south orientation. The LF wave energy of the northern branch from the Atlantic Ocean disperses to Northeast China, which excites the downstream disturbance wave train. The corresponding LF positive vorticity enhances and moves eastward, leading to the formation of deep EAT. The enhanced subsidence motion behind the EAT leads to SH strengthening. The cold advection related to the northeast cold vortex is the main thermal factor causing the local temperature to decrease. The Scandinavian Peninsula is the primary cold air source, and the Laptev Sea is the secondary one, with cold air from the former along northwest path via the West Siberian Plain and Lake Baikal, and from the latter along the northern path via the Central Siberian Plateau, both converging towards Northeast China. Full article
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<p>The regional average frequency of the winter RSCEs in Northeast China from 1980 to 2021. Unit: number of occurrences.</p>
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<p>(<b>a</b>) Morlet wavelet energy spectrum of the regional average daily minimum temperature in the winter of 2020 in Northeast China (contours). The shaded area is significant at the 0.1 level. The area between the red vertical lines is winter, while the red horizontal lines correspond to 10 d, 20 d, 30 d, 60 d, and 90 d, respectively. (<b>b</b>) The above minimum temperature series (bar, °C) and its 10–20 d components (solid line, °C). The interval between the two vertical lines denotes the strong cooling process, with the 3–7 phase.</p>
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<p>The 10–20 d (<b>a1</b>–<b>a3</b>) 300 hPa zonal wind fields (shaded, m/s), (<b>b1</b>–<b>b3</b>) 500 hPa geopotential height fields (shaded, gpm; contours: unfiltered), (<b>c1</b>–<b>c3</b>) 850 hPa wind (vectors, m/s) and temperature fields (shaded, <span class="html-italic">K</span>), and (<b>d1</b>–<b>d3</b>) SLP fields (shaded, hPa; contours: unfiltered) composited by 60 RSCEs at phases 3, 5, and 7, respectively. The dotted areas are significant at the 0.01 level. “+” (“−”) indicates a positive (negative) anomaly.</p>
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<p>(<b>a</b>–<b>c</b>) The 850 hPa 10–20 d isobaric PV (shaded, <math display="inline"><semantics> <mrow> <mi>P</mi> <mi>V</mi> <mi>U</mi> </mrow> </semantics></math>) fields composited by 60 RSCEs at phases 3, 5, and 7, respectively. The dotted areas are significant at the 0.01 level. “+” (“−”) indicates a positive (negative) anomaly.</p>
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<p>Height–longitude profiles of meridional average 10–20 d (<b>a</b>–<b>c</b>) vorticity (shaded, <math display="inline"><semantics> <msup> <mn>10</mn> <mrow> <mo>−</mo> <mn>6</mn> </mrow> </msup> </semantics></math> s<sup>−1</sup>) and (<b>d</b>–<b>f</b>) divergence (shaded, 10<sup>−7</sup> s<sup>−1</sup>) along the latitudes 50–70° N, 50–60° N and 40–55° N at phases 3, 5, and 7, respectively. The vector is 10–20 d vertical zonal circulation (m/s). The dotted areas are significant at the 0.01 level.</p>
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<p>(<b>a</b>–<b>c</b>) 300 hPa 10–20 d horizontal WAF (vector, m<sup>2</sup>/s<sup>2</sup>) and its divergence (shaded, <math display="inline"><semantics> <msup> <mn>10</mn> <mrow> <mo>−</mo> <mn>8</mn> </mrow> </msup> </semantics></math> m/s<sup>2</sup>) and 10–20 d geostrophic stream function (contours, <math display="inline"><semantics> <msup> <mn>10</mn> <mn>5</mn> </msup> </semantics></math> m<sup>2</sup>s) composited by 60 RSCEs at phases 3, 5, and 7, respectively. The dotted areas are significant at the 0.01 level.</p>
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<p>The 850 hPa 10–20 d (<b>a</b>–<b>c</b>) local temperature change, (<b>d</b>–<b>f</b>) temperature advection, (<b>g</b>–<b>i</b>) vertical motion adiabatic change, and (<b>j</b>–<b>l</b>) diabatic heating composited by 60 RSCEs at phases 3, 5, and 7, respectively. Unit: K/day, the dotted areas are significant at the 0.01 level.</p>
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<p>The 850 hPa 10–20 d thermodynamic energy equation evolution of each term’s regional mean in Northeast China at phases 3–7.</p>
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<p>(<b>a</b>) Weighted K-means clustering of stations in Northeast China; the “▼” are for four representative stations (S1, S2, S3, and S4) and the “★” are for the cluster centers. (<b>b</b>) The cold air HYSPLIT backward trajectory simulation for 60 RSCEs at four representative stations in Northeast China. The percentage represents the contribution ratio.</p>
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21 pages, 5612 KiB  
Article
Beyond Temperature Peaks: The Growing Persistence and Intensity of Tmin and Tmax Heatwaves in Portugal’s Changing Climate (1980/1981–2022/2023)
by Luis Angel Espinosa, Maria Manuela Portela and Nikte Ocampo-Guerrero
Atmosphere 2024, 15(12), 1485; https://doi.org/10.3390/atmos15121485 (registering DOI) - 12 Dec 2024
Viewed by 276
Abstract
This study examines the trends in heatwave characteristics across mainland Portugal from 1980/1981 to 2022/2023, utilising ERA5-Land reanalysis data. To achieve this, the study applies the Heatwave Magnitude Index (HWMI) to identify heatwave days for minimum (Tmin) and maximum (Tmax [...] Read more.
This study examines the trends in heatwave characteristics across mainland Portugal from 1980/1981 to 2022/2023, utilising ERA5-Land reanalysis data. To achieve this, the study applies the Heatwave Magnitude Index (HWMI) to identify heatwave days for minimum (Tmin) and maximum (Tmax) temperatures across 15 grid-points representing Portugal’s diverse geography and climate. Three key annual parameters are analysed: the number of heatwave days (ANDH), the average temperature during heatwaves (AATW), and the intensity of heatwave events (AIHD). Results reveal a consistent increase in heatwave persistence throughout mainland Portugal, with more pronounced trends observed for Tmax compared to Tmin. ANDH Tmin shows upward trends across all grid-points, with increases ranging from 0.8 to 4.2 days per decade. ANDH Tmax exhibits even more significant increases, with 11 out of 15 grid-points showing statistically significant rises, ranging from 2.2 to 4.4 days per decade. Coastal areas, particularly in the south, demonstrate the most substantial increases in heatwave persistence. The intensity of heatwaves, as measured by AIHD, also shows positive trends across all grid-points for both Tmin and Tmax, with southern locations experiencing the most significant increases. The study also discusses decadal trends in annual averages of Tmin and Tmax, as well as extreme measures such as annual minimum (AMIN) and annual maximum (AMAX), daily temperatures spatially represented across mainland Portugal. These analyses reveal widespread warming trends, with more pronounced increases in Tmax compared to Tmin. The AMIN and AMAX trends further corroborate the overall warming pattern from the heatwave analyses, with notable spatial variations observed. The findings indicate a substantial worsening in the occurrence, duration, and intensity of heatwave events. This increased persistence of heatwaves, especially evident from the early 2000s onwards, suggests a potential climate regime shift in mainland Portugal. The results underscore the need for adaptive strategies to address the growing challenges posed by more frequent and intense heatwaves in the region. Full article
(This article belongs to the Special Issue New Perspectives in Hydrological Extremes)
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Figure 1

Figure 1
<p>Geographical distribution and temperature data across mainland Portugal: (<b>a</b>) topography, highlighting some provinces, and the ERA5-Land 1012 grid-points used for analysis; (<b>b</b>) average of minimum daily temperatures, T<sub>min</sub>, over the 43 hydrological years from 1980/1981 to 2022/2023, with the names of the 15 focal grid-points indicated; (<b>c</b>) average of maximum daily temperatures, T<sub>max</sub>, for the same period, with the corresponding location codes shown. Maps in (<b>b</b>,<b>c</b>) were produced using the 1012 grid-points and Inverse Distance Weighting with a power of 2 (IDW2).</p>
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<p>Averages of annual minimum daily temperatures from 1980/1981 to 2022/2023: (<b>a</b>) for the minimum temperatures (AMIN T<sub>min</sub>), with the names of the 15 focal Portuguese locations indicated; (<b>b</b>) for the maximum temperatures (AMIN T<sub>max</sub>) for the same period, with corresponding location codes shown. Maps were produced using the 1012 grid-points and IDW2.</p>
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<p>Averages of annual maximum daily temperatures from 1980/1981 to 2022/2023: (<b>a</b>) for the minimum temperatures (AMAX T<sub>min</sub>), with the names of the 15 focal Portuguese locations indicated; (<b>b</b>) for the maximum temperatures (AMAX T<sub>max</sub>) for the same period, with corresponding location codes shown. Maps were produced using the 1012 grid-points and IDW2.</p>
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<p>Heatwave thresholds (<math display="inline"><semantics> <msub> <mi>A</mi> <mi>d</mi> </msub> </semantics></math>) for (<b>a</b>) T<sub>min</sub> and (<b>b</b>) T<sub>max</sub> across 15 focal grid-points in mainland Portugal. Thresholds were calculated as the 90th percentile of daily temperatures for the hydrological years 1980/1981 to 2022/2023. The grid-points, listed from north to south and west to east, include (codes between brackets): Bragança (BGCA), Braga (BRGA), Porto (PRTO), Aveiro (AVRO), Guarda (GRDA), Coimbra (CMBR), Castelo Branco (CABO), Nazaré (NZRE), Portalegre (PTLG), Santarém (STRM), Lisbon (LISB), Évora (EVRA), Beja (BEJA), Lagos (LGOS), and Faro (FARO).</p>
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<p>Temporal evolution of annual number of heatwave days (ANDH) for (<b>a</b>) T<sub>min</sub> and (<b>b</b>) T<sub>max</sub> across 15 focal grid-points in mainland Portugal, based on the Mann-Kendall-Sneyers (MKS) test. The progressive statistic <math display="inline"><semantics> <mrow> <mi>u</mi> <mo>(</mo> <mi>t</mi> <mo>)</mo> </mrow> </semantics></math> is shown, with Kendall’s normalised tau on the <span class="html-italic">y</span>-axis. Tau values outside the range ±1.96 indicate statistically significant trends at the <math display="inline"><semantics> <mrow> <mn>95</mn> <mo>%</mo> </mrow> </semantics></math> confidence level.</p>
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<p>Temporal evolution of annual average temperature during heatwaves (AATW) for (<b>a</b>) T<sub>min</sub> and (<b>b</b>) T<sub>max</sub> across 15 focal grid-points in mainland Portugal, based on the Mann-Kendall-Sneyers (MKS) test. The progressive statistic <math display="inline"><semantics> <mrow> <mi>u</mi> <mo>(</mo> <mi>t</mi> <mo>)</mo> </mrow> </semantics></math> is shown, with Kendall’s normalised tau on the <span class="html-italic">y</span>-axis. Tau values outside the range ±1.96 indicate statistically significant trends at the <math display="inline"><semantics> <mrow> <mn>95</mn> <mo>%</mo> </mrow> </semantics></math> confidence level.</p>
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<p>Temporal evolution of annual intensity of heatwave events (AIHD) for (<b>a</b>) T<sub>min</sub> and (<b>b</b>) T<sub>max</sub> across 15 focal grid-points in mainland Portugal, based on the Mann-Kendall-Sneyers (MKS) test. The progressive statistic <math display="inline"><semantics> <mrow> <mi>u</mi> <mo>(</mo> <mi>t</mi> <mo>)</mo> </mrow> </semantics></math> is shown, with Kendall’s normalised tau on the <span class="html-italic">y</span>-axis. Tau values outside the range ±1.96 indicate statistically significant trends at the <math display="inline"><semantics> <mrow> <mn>95</mn> <mo>%</mo> </mrow> </semantics></math> confidence level.</p>
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<p>Decadal trends based on Sen’s slope and 43 annual means, from 1980/1981 to 2022/2023, of (<b>a</b>) T<sub>min</sub>, with the names of 15 focal grid-points indicated; and (<b>b</b>) T<sub>max</sub>, with corresponding region codes shown. Maps were produced using 1012 grid-points and IDW2 interpolation.</p>
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<p>Decadal trends based on Sen’s slope and 43 annual values, from 1980/1981 to 2022/2023, in (<b>a</b>) AMIN T<sub>min</sub>, with the names of 15 focal grid-points indicated; and (<b>b</b>) AMIN T<sub>max</sub>, with corresponding region codes shown. Maps were produced using 1012 grid-points and IDW2 interpolation.</p>
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<p>Decadal trends based on Sen’s and the 43 annual values, from 1980/1981 to 2022/2023, in (<b>a</b>) AMAX T<sub>min</sub>, with the names of 15 focal grid-points indicated; and (<b>b</b>) AMAX T<sub>max</sub>, with corresponding region codes shown. Maps were produced using 1012 grid-points and IDW2 interpolation.</p>
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22 pages, 18686 KiB  
Article
An Idealized Cloud-Resolving Modeling Study on Rainfall in Taiwan Under Uniform Northeasterly Flow in Winter, Part I: Effects of Wind Direction, Speed, and Moisture Amount
by Chung-Chieh Wang, Chun-Hsien Li, Shin-Yi Huang and Chih-Sheng Chang
Atmosphere 2024, 15(12), 1484; https://doi.org/10.3390/atmos15121484 - 12 Dec 2024
Viewed by 300
Abstract
This study performs idealized simulations of rainfall in Taiwan in a winter monsoon regime under different wind direction (Wd; every 15° from 0° to 90°), speed (Ws; 12, 8, and 4 m s−1), and relative [...] Read more.
This study performs idealized simulations of rainfall in Taiwan in a winter monsoon regime under different wind direction (Wd; every 15° from 0° to 90°), speed (Ws; 12, 8, and 4 m s−1), and relative humidity (RH; 80, 70, and 60%) combinations at low levels, based on a simplified mean sounding profile from observations during the event over 20–24 November 2020. Thus, at a horizontal grid size of 2 km, a total of 7 × 3 × 3 = 63 runs are performed and the aim is to investigate the response in daily rainfall in northern Taiwan to these three parameters. The model results from the closest combination are verified against the observed rainfall both during the reference event and in several historical cases with reasonable agreement, indicating the usefulness of the approach, albeit with some limitations. From the experiments, our main findings can be summarized as below. First and foremost, with Ws = 12 m s−1 and RH = 80%, when the prescribed Wd changes from 0° (northerly) to 90° (easterly) gradually, the main rainfall areas shift from northern to northeastern Taiwan, with local maxima at the northern tip, northeastern tip of Taiwan, and near Suao (at the end of the Central Mountain Range) in response, indicating topographic uplifting for rainfall production. At a larger impinging angle, the Suao area tends to receive the most daily rainfall and can exceed 300 mm at Wd of about 75°–80°. Second, when Ws decreases to 8 m s−1, the general rainfall regions often remain similar but the amounts become lower, especially at local maxima. The peak amount near Suao is only about 100 mm. At weak wind of Ws = 4 m s−1, only moderate rainfall of 20 mm or below can be produced in Taiwan, and the local centers become not discernable. Third, when RH is lowered, the rainfall in northern Taiwan decreases significantly, especially along and near the coast under weaker winds coming from smaller angles. At RH = 70%, a higher accumulation (≥100 mm or so) near Suao is only possible with Wd ≥ about 55° at Ws = 12 m s−1 or when Wd ≥ 70° at Ws = 8 m s−1. At RH = 60%, the rainfall in northern Taiwan (and on the entire island) further decreases, again more evidently in cases with smaller Wd and Ws values. Full article
(This article belongs to the Special Issue Island Effects on Weather and Climate)
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Figure 1
<p>(<b>a</b>) A map surrounding Taiwan with topography (m, gray shades), model simulation domain (thick dashed), and region to compute the mean sounding profile upstream from Taiwan (dotted box, over 25.0–27.5° N, 122.5–125.0° E). (<b>b</b>) Enlarged map showing the model domain and detailed topography (m, gray shades), with locations of Pengchiayu Islet (triangle), Guishan Island, and averaging box for upstream wind direction near Taiwan in experiments (thick box, over 25.75–26.25° N, 122.5–123.0° E).</p>
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<p>Rose diagram of surface winds at (<b>a</b>) Pengchiayu and (<b>b</b>) Guishan Island (locations shown in <a href="#atmosphere-15-01484-f001" class="html-fig">Figure 1</a>b), obtained from hourly data over September to February, 2011–2020, excluding dates under the influence of typhoon or front. Colors indicate wind-speed ranges (m s<sup>−1</sup>, legend) and each concentric ring represents 2.6% in (<b>a</b>) and 2.8% in (<b>b</b>), respectively. The total sample size is 26,976.</p>
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<p>(<b>a</b>) The topography (m, color), locations of rain gauges (blue dots) in Taiwan, and the domain for the calculation of the Similarity Skill Score (red area, see <a href="#sec2dot4-atmosphere-15-01484" class="html-sec">Section 2.4</a> for details). The two major mountain ranges are also labeled. (<b>b</b>) Enlarged and detailed topography (m, color) in northern Taiwan, with Yilan County and the location of Suao (scarlet dot) marked.</p>
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<p>The CWA surface weather charts at 0000 UTC of (<b>a</b>–<b>d</b>) 21–24 November 2020, respectively. Isobars of mean sea-level pressure are analyzed every 4 hPa (solid, thickened every 20 hPa) and at 2 hPa intervals (dashed). Surface fronts and high/low centers are also marked (with moving speed/direction labeled where needed).</p>
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<p>As in <a href="#atmosphere-15-01484-f004" class="html-fig">Figure 4</a>, except at 850 hPa at 0000 UTC of (<b>a</b>) 21 and (<b>b</b>) 24 November 2020, respectively. Geopotential heights are analyzed every 30 gpm (solid, thickened every 60 gpm), isotherms (°C, red dashed) every 3 °C, and high/low centers and warm regions are also labeled if needed.</p>
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<p>Mean vertical profiles of temperature <span class="html-italic">T</span> (°C, red curve), dew-point temperature <span class="html-italic">T<sub>d</sub></span> (°C, blue curve), and horizontal wind (kt, barbs on the right side) in the Skew <span class="html-italic">T</span>-log <span class="html-italic">p</span> diagram, obtained from NCEP analyses (<b>a</b>) before and (<b>b</b>) after smoothing (see text for detail).</p>
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<p>Mean vertical profiles of (<b>a</b>) horizontal wind speed (<span class="html-italic">W<sub>s</sub></span>, red) and the zonal (<span class="html-italic">u</span>, green) and meridional component (<span class="html-italic">v</span>, blue, all in m s<sup>−1</sup>), (<b>b</b>) horizontal wind direction (<span class="html-italic">W<sub>d</sub></span>, °), and (<b>c</b>) relative humidity (<span class="html-italic">RH</span>, %, curve with open dots, scale at bottom) and specific humidity (<span class="html-italic">q<sub>v</sub></span>, g kg<sup>−1</sup>, curve with squares, scale on top) obtained from NCEP analyses before smoothing (i.e., data as in <a href="#atmosphere-15-01484-f006" class="html-fig">Figure 6</a>a). (<b>d</b>–<b>f</b>) As in (<b>a</b>–<b>c</b>), except after smoothing (i.e., data as in <a href="#atmosphere-15-01484-f006" class="html-fig">Figure 6</a>b). Additional wind speeds used in the model (4 and 8 m s<sup>–1</sup> at the surface) are also plotted in (<b>d</b>), selected wind directions (30°, 60°, and 90°) plotted in (<b>e</b>), and additional <span class="html-italic">RH</span> (60% and 70% at the surface) plotted in (<b>f</b>) without <span class="html-italic">q<sub>v</sub></span>, respectively.</p>
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<p>Comparison between observed (top row, produced and provided by the CWA) and model-simulated (bottom row) daily rainfall distributions (mm, color) in LST over Taiwan for the period of 20–24 November 2020. For each panel, the combinations of <span class="html-italic">RH</span>, <span class="html-italic">W<sub>s</sub></span>, and <span class="html-italic">W<sub>d</sub></span> are labeled on the top. In addition, the duration of northeasterly flow on each day (Δ<span class="html-italic">t</span>, in h) for observation and the values of RMSE, SSS, and Bias for model rainfall in northern Taiwan are also given.</p>
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<p>Selected examples of column-maximum radar reflectivity (dBZ, scale to the right) near Taiwan at 0500 LST on 20, 0900 LST on 21, 1130 and 2200 LST on 23, and 1100 LST on 24 November 2020, respectively (from left to right), during the reference case, with terrain also shown (original figures produced and provided by the CWA).</p>
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<p>Total daily rainfall distribution (mm, scale on the right) and streamlines of time-averaged surface flow at 10 m height over Taiwan from 0000 to 2400 LST (<span class="html-italic">t</span> = 18–42 h) in the 7 × 3 = 21 experiments of different initial wind direction (every 15° from 0° to 90°, columns, labeled on top) and speed (12, 8, and 4 m s<sup>−1</sup>, rows, labeled on the left), respectively, at the setting of <span class="html-italic">RH</span> = 80% at 1000 hPa near the surface (upper left). Inside each panel, the wind direction upstream from northeastern Taiwan during the accumulation period is also given (°).</p>
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<p>As in <a href="#atmosphere-15-01484-f010" class="html-fig">Figure 10</a>, except for the 21 experiments at the setting of <span class="html-italic">RH</span> = 70% at 1000 hPa.</p>
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<p>As in <a href="#atmosphere-15-01484-f010" class="html-fig">Figure 10</a>, except for the 21 experiments at the setting of <span class="html-italic">RH</span> = 60% at 1000 hPa.</p>
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<p>As in <a href="#atmosphere-15-01484-f008" class="html-fig">Figure 8</a>, except for comparison between observed (source: CWA) and model-simulated daily rainfall distributions (mm, color) in five selected historical cases on (from left to right) 2 November 2014, 25 November 2016, 18 December 2017, 30 December 2017, and 30 January 2018, respectively. For all cases, the duration of northeasterly flow (Δ<span class="html-italic">t</span>) is 24 h and not labeled.</p>
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19 pages, 4346 KiB  
Article
Experimental Study on the Change in Freezing Temperature During the Remediation of Pb-Contaminated Soils with Biochar
by Shanbo Han, Wei Cao, Yaling Chou and Erxing Peng
Atmosphere 2024, 15(12), 1483; https://doi.org/10.3390/atmos15121483 - 12 Dec 2024
Viewed by 248
Abstract
In the remediation process of heavily metal-contaminated soil, biochar can change the ion content and soil structure, significantly impacting soil freezing. This experiment used freezing ambient temperature, water (W) content, heavy metal (M) contents, and biochar (BC) contents as factors affecting soil freezing. [...] Read more.
In the remediation process of heavily metal-contaminated soil, biochar can change the ion content and soil structure, significantly impacting soil freezing. This experiment used freezing ambient temperature, water (W) content, heavy metal (M) contents, and biochar (BC) contents as factors affecting soil freezing. The test soil was manually compacted in a homemade acrylic device to achieve a compaction level of 90%. The temperature changes of the soil during low-temperature freezing were monitored through thermometry experiments. The results indicated that soil freezing temperature decreased with increasing heavy metal and biochar contents and increased with increasing initial water content and freezing ambient temperature. Multiple freeze–thaw cycles revealed the interaction between biochar and heavy metals. The effects of biochar on the freezing temperature of soil with different heavy metal contents were different; in the soil with the same heavy metal content, 3% biochar contents had little effect on the freezing temperature of heavy metal-polluted soil, and 5% and 7% biochar contents significantly improved the freezing resistance of the soil. Freeze–thaw cycling had little effect on the soil’s microporous structure, resulting in minimal changes in soil freezing temperatures after seven cycles. Correlation analyses of heavy metals, water content, and biochar revealed that the effects of these factors on freezing temperature were in the order of heavy metals > water > biochar. The composite freezing temperature of biochar and heavy metal overlaps well. The initial freezing temperature of the soil was used to predict the unfrozen water in the soil. The prediction results showed that biochar increased the content of unfrozen water in the soil. Full article
(This article belongs to the Section Climatology)
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Figure 1
<p>Soil sample collection.</p>
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<p>Compaction and freezing of soil samples. (<b>a</b>) Soil sample compaction. (<b>b</b>) Soil sample freezing.</p>
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<p>Effect of different lead contents on soil freezing temperature.</p>
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<p>Effect of different lead contents on soil freezing temperature under freeze–thaw action. (<b>a</b>) BC = 0%, W = 15%. (<b>a<sub>1</sub></b>) First freeze, (<b>a<sub>2</sub></b>) second freezing, (<b>a<sub>3</sub></b>) third freezing.</p>
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<p>Effect of different lead contents on soil freezing temperature under freeze–thaw action. (<b>a</b>) BC = 0%, W = 15%. (<b>a<sub>1</sub></b>) First freeze, (<b>a<sub>2</sub></b>) second freezing, (<b>a<sub>3</sub></b>) third freezing.</p>
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<p>Effects of different biochar content on soil freezing temperature. (<b>a</b>) M = 0.1–0.2%, (<b>b</b>) M = 0.3–0.5%, (<b>c</b>) M = 1–2%.</p>
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<p>Effect of biochar content on freezing temperature of different lead-contaminated soils under freeze–thaw cycle. (<b>a</b>) M = 0%, W = 15%, (<b>a<sub>1</sub></b>) first freeze, (<b>a<sub>2</sub></b>) second freeze, (<b>a<sub>3</sub></b>) third freeze, (<b>b</b>) M = 0.5%, W = 15%, (<b>b<sub>1</sub></b>) first freeze, (<b>b<sub>2</sub></b>) second freeze, (<b>b<sub>3</sub></b>) third freeze, (<b>c</b>) M = 1%, W = 15%, (<b>c<sub>1</sub></b>) first freeze, (<b>c<sub>2</sub></b>) second freeze, (<b>c<sub>3</sub></b>) third freeze.</p>
Full article ">Figure 6 Cont.
<p>Effect of biochar content on freezing temperature of different lead-contaminated soils under freeze–thaw cycle. (<b>a</b>) M = 0%, W = 15%, (<b>a<sub>1</sub></b>) first freeze, (<b>a<sub>2</sub></b>) second freeze, (<b>a<sub>3</sub></b>) third freeze, (<b>b</b>) M = 0.5%, W = 15%, (<b>b<sub>1</sub></b>) first freeze, (<b>b<sub>2</sub></b>) second freeze, (<b>b<sub>3</sub></b>) third freeze, (<b>c</b>) M = 1%, W = 15%, (<b>c<sub>1</sub></b>) first freeze, (<b>c<sub>2</sub></b>) second freeze, (<b>c<sub>3</sub></b>) third freeze.</p>
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<p>Correlation analysis of biochar, heavy metal, and water on soil freezing temperature.</p>
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<p>Effect of initial water content on freezing temperature of different soils. (<b>a</b>) M = 0–0.2%, (<b>b</b>) M = 0.3–0.5%, (<b>c</b>) M = 1–2%.</p>
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<p>Changing law of soil freezing temperature under different adverse temperature environments. (<b>a</b>) W = 15%, (<b>b</b>) W = 20%, (<b>c</b>) W = 25%.</p>
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<p>Calculated relationships for unfrozen water in soils with different biochar contents.</p>
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28 pages, 19078 KiB  
Article
Analysis of PM2.5 Pollution Transport Characteristics and Potential Sources in Four Chinese Megacities During 2022: Seasonal Variations
by Kun Mao, Yuan Yao, Kun Wang, Chen Liu, Guangmin Tang, Shumin Feng, Yue Shen, Anhua Ju, Hao Zhou and Zhiyu Li
Atmosphere 2024, 15(12), 1482; https://doi.org/10.3390/atmos15121482 - 12 Dec 2024
Viewed by 406
Abstract
Atmospheric particulate pollution in China’s megacities has heightened public concern over air quality, highlighting the need for precise identification of urban pollution characteristics and pollutant transport mechanisms to enable effective control and mitigation. In this study, a new method combing the High Accuracy [...] Read more.
Atmospheric particulate pollution in China’s megacities has heightened public concern over air quality, highlighting the need for precise identification of urban pollution characteristics and pollutant transport mechanisms to enable effective control and mitigation. In this study, a new method combing the High Accuracy Surface Modeling (HASM) and Multiscale Geographically Weighted Regression (MGWR) was proposed to derive seasonal high spatial resolution PM2.5 concentrations. The Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) was applied to analyze the seasonal spatial variations, transport pathways, and potential sources of PM2.5 concentrations across China’s four megacities: Beijing, Shanghai, Xi’an, and Chengdu. The result indicates that: (1) the proposed method outperformed Kriging, inverse distance weighting (IDW), and HASM, with coefficient of determination values ranging from 0.91 to 0.94, and root mean square error values ranging from 1.98 to 2.43 µg/m3, respectively; (2) all cities show a similar seasonal pattern, with PM2.5 concentrations highest in winter, followed by spring, autumn, and summer; Beijing has higher concentrations in the south, Shanghai and Xi’an in the west, and Chengdu in central urban areas, decreasing toward the rural area; (3) potential source contribution function and concentration weighted trajectory analysis indicate that Beijing’s main potential PM2.5 sources are in Hebei Province (during winter, spring, and autumn), Shanghai’s are in the Yellow Sea and the East China Sea, Xi’an’s are in Southern Shaanxi Province, and Chengdu’s are in Northeastern and Southern Sichuan Province, with all cities experiencing higher impacts in winter; (4) there is a negative correlation between precipitation, air temperature, and seasonal PM2.5 levels, with anthropogenic emissions sources such as industry combustion, power plants, residential combustion, and transportation significantly impact on seasonal PM2.5 pollution. Full article
(This article belongs to the Section Air Quality)
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<p>Location of the Beijing, Shanghai, Xi’an, and Chengdu in China.</p>
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<p>Flowchart of the proposed method downscaling process.</p>
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<p>Interpolation accuracy validation of PM<sub>2.5</sub> concentrations for the four megacities. (<b>a</b>) Beijing. (<b>b</b>) Shanghai. (<b>c</b>) Xi’an. (<b>d</b>) Chengdu.</p>
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<p>Seasonal PM<sub>2.5</sub> concentration surfaces for the four megacities predicted by the proposed method.</p>
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<p>Seasonal cluster–mean backward trajectories arriving in Beijing during 2022, showing the main transport pathways of air masses (II: Inner Mongolia Autonomous Region, XVIII: Hebei Province). (<b>a</b>) Spring. (<b>b</b>) Summer. (<b>c</b>) Autumn. (<b>d</b>) Winter.</p>
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<p>Seasonal cluster–mean backward trajectories arriving in Shanghai in 2022, showing the main transport pathways of air masses (II: Inner Mongolia Autonomous Region, III: Liaoning Province, IV: Shandong Province, VII: Jiangsu Province, XIII: Zhejiang Province, XIV: Fujian Province, XV: Anhui Province, XVIII: Hebei Province). (<b>a</b>) Spring. (<b>b</b>) Summer. (<b>c</b>) Autumn. (<b>d</b>) Winter.</p>
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<p>Seasonal cluster–mean backward trajectories arriving in Shanghai in 2022, showing the main transport pathways of air masses (II: Inner Mongolia Autonomous Region, III: Liaoning Province, IV: Shandong Province, VII: Jiangsu Province, XIII: Zhejiang Province, XIV: Fujian Province, XV: Anhui Province, XVIII: Hebei Province). (<b>a</b>) Spring. (<b>b</b>) Summer. (<b>c</b>) Autumn. (<b>d</b>) Winter.</p>
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<p>Seasonal cluster–mean backward trajectories arriving in Xi’an in 2022, showing the main transport pathways of air masses (II: Inner Mongolia Autonomous Region, V: Shaanxi Province, VI: Henan Province, VIII: Gansu Province, X: Hubei Province, XI: Chongqing City, XVIII: Xinjiang Uygur Autonomous Region). (<b>a</b>) Spring. (<b>b</b>) Summer. (<b>c</b>) Autumn. (<b>d</b>) Winter.</p>
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<p>Seasonal cluster–mean backward trajectories arriving in Chengdu in 2022, showing the main transport pathways of air masses (V: Shaanxi Province, VIII: Gansu Province, IX: Sichuan Province, XI: Chongqing City, XXI: Tibet Autonomous Region, XXII: Guizhou Province). (<b>a</b>) Spring. (<b>b</b>) Summer. (<b>c</b>) Autumn. (<b>d</b>) Winter.</p>
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<p>Source identification for PM<sub>2.5</sub> over Beijing, Shanghai, Xi’an, and Chengdu using PSCF analysis during four seasons in 2022.</p>
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<p>Source identification for PM<sub>2.5</sub> over Beijing, Shanghai, Xi’an, and Chengdu using CWT analysis during four seasons in 2022.</p>
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<p>Source identification for PM<sub>2.5</sub> over Beijing, Shanghai, Xi’an, and Chengdu using CWT analysis during four seasons in 2022.</p>
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<p>Air temperature distribution in the primary pollution transport pathway areas for four study areas during three seasons in 2022.</p>
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<p>Precipitation distribution in the primary pollution transport pathway areas for four study areas during three seasons in 2022.</p>
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<p>Precipitation distribution in the primary pollution transport pathway areas for four study areas during three seasons in 2022.</p>
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18 pages, 2383 KiB  
Article
An AutoML-Powered Analysis Framework for Forest Fire Forecasting: Adapting to Climate Change Dynamics
by Shuo Zhang and Mengya Pan
Atmosphere 2024, 15(12), 1481; https://doi.org/10.3390/atmos15121481 - 11 Dec 2024
Viewed by 400
Abstract
Wildfires pose a serious threat to ecosystems and human safety, and with the backdrop of global climate change, the prediction of forest fires has become increasingly important. Traditional machine learning methods face challenges in forest fire prediction, such as difficulty identifying feature parameters, [...] Read more.
Wildfires pose a serious threat to ecosystems and human safety, and with the backdrop of global climate change, the prediction of forest fires has become increasingly important. Traditional machine learning methods face challenges in forest fire prediction, such as difficulty identifying feature parameters, manual intervention in model selection, and hyperparameter tuning, which affect prediction accuracy and efficiency. This study proposes an analytical framework for forest fire prediction based on Automated Machine Learning (AutoML) technology to address the challenges traditional machine learning methods face in forest fire prediction. We collected meteorological, topographical, and vegetation data from Guangxi Province, with meteorological data covering 1994 to 2023, providing comprehensive background information for our prediction model. Using the prediction model, which was constructed with the AutoGluon framework, the experimental results indicate that models under the AutoGluon framework (e.g., KNeighborsDist classifier) significantly outperform traditional machine learning models in terms of accuracy, precision, recall, and F1-Score, with the highest accuracy rate reaching 0.960. Model error analysis shows that models under the AutoGluon framework perform better in error control. This study provides an efficient and accurate method for forest fire prediction, which is of great significance for decision-making in forest fire management and for protecting forest resources and ecological security. Full article
(This article belongs to the Special Issue Forest Ecosystems in a Changing Climate)
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<p>Number of forest fires and burned areas in China from 2002 to 2023.</p>
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<p>Number of Forest fires and burned areas in Guangxi from 2002 to 2023.</p>
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<p>Vegetation type distribution map of Guangxi Province.</p>
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<p>Climate change in Guangxi Province, 1994–2003.</p>
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<p>Pearson correlation coefficient of variables in the dataset.</p>
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<p>Pearson correlation coefficient of variables in the dataset.</p>
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<p>Multi-layer overlay integration strategy.</p>
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<p>Predicted versus true values for different models.</p>
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<p>Distribution of prediction error of the AutoML models.</p>
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23 pages, 1892 KiB  
Review
Are Agroecosystem Services Under Threat? Examining the Influence of Climate Externalities on Ecosystem Stability
by Temidayo Olowoyeye, Gideon Abegunrin and Mariusz Sojka
Atmosphere 2024, 15(12), 1480; https://doi.org/10.3390/atmos15121480 - 11 Dec 2024
Viewed by 310
Abstract
This study examines the impacts of climate-induced externalities on the stability of agroecosystems and the ecosystem services they provide. Using the PRISMA approach, we review literature published from 2015 to 2024. The study identifies how extreme weather events such as droughts, floods, heatwaves, [...] Read more.
This study examines the impacts of climate-induced externalities on the stability of agroecosystems and the ecosystem services they provide. Using the PRISMA approach, we review literature published from 2015 to 2024. The study identifies how extreme weather events such as droughts, floods, heatwaves, and altered precipitation patterns disrupt the provisioning, regulating, and supporting services critical to food security, soil fertility, water purification, and biodiversity. Our findings show a continued increase in climate extremes, raising concerns about food security, environmental resilience, and socio-economic stability. It also reveals that regions dependent on rain-fed agriculture, such as parts of Africa, Asia, and the Mediterranean, are particularly vulnerable to these stressors. Adaptation strategies, including conservation agriculture, crop diversification, agroforestry, and improved water management, are identified as crucial for mitigating these impacts. This study emphasises the importance of proactive, policy-driven approaches to foster climate resilience, support agroecosystem productivity, and secure ecosystem services critical to human well-being and environmental health. Full article
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<p>Conceptual framework for the review synthesis.</p>
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<p>PRISMA flow diagram showing the process and shape of the systematic literature review.</p>
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<p>Text analysis of selected articles.</p>
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<p>Frequency of primary keywords.</p>
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<p>Map showing the distribution of climate externalities research, highlighting regions with reported extreme climate threats to environmental stability based on papers included in the review.</p>
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16 pages, 2182 KiB  
Article
Enhancements of Triethanolamine CO2 Absorption Rate and Degradation in the Presence of Nickel Nanoparticles Catalysts
by Harold W. Orendi, Kevin Joby and Lidija Šiller
Atmosphere 2024, 15(12), 1479; https://doi.org/10.3390/atmos15121479 - 11 Dec 2024
Viewed by 274
Abstract
Here, the catalytic and degradation effect of nickel nanoparticles (NiNPs) on triethanolamine (TEA) with CO2 at 20 °C and 50 °C and a range of TEA concentrations (3–30 wt%) was studied. We show that TEA absorption rate of CO2 can be [...] Read more.
Here, the catalytic and degradation effect of nickel nanoparticles (NiNPs) on triethanolamine (TEA) with CO2 at 20 °C and 50 °C and a range of TEA concentrations (3–30 wt%) was studied. We show that TEA absorption rate of CO2 can be enhanced with NiNPs, the maximum enhancement was 8.3% when compared to a control solution found at 50 °C with 30 wt% TEA alone. Additionally, the time for TEA to be fully loaded with CO2 is reduced; compared to the control, NiNPs enhanced solutions were up to 26.3% faster. Also, to the best of our knowledge, this is the first time the degradation of TEA with NiNPs has been studied. TEA was subject to both oxygen (30 wt%, 55 °C, 0.35 L/min of air, 0.4 molCO2/molTEA, 7.5 mL/min of CO2) and thermal degradation with and without NiNPs (30 wt%, 0.5 molCO2/molTEA, 135 °C). In both degradation experiments, surprisingly, there was no significant difference in TEA degradation in the presence of NiNPs. At high temperature (135 °C), the solution lost 19.2% and 20.3% of the original TEA, with and without NiNPs, respectively. In the presence of oxygen, the solution lost 30.5% and 33.6% of the original TEA, with and without NiNPs, respectively. This indicates that TEA or its mixture with other amines and NiNPs could improve post-combustion CO2 capture. Full article
(This article belongs to the Special Issue Advances in CO2 Capture and Absorption)
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<p>Schematic of the reaction mechanism of hydration of CO<sub>2</sub> by NiNPs, adopted from [<a href="#B17-atmosphere-15-01479" class="html-bibr">17</a>,<a href="#B29-atmosphere-15-01479" class="html-bibr">29</a>].</p>
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<p>Diagram of CO<sub>2</sub> loading apparatus used for the CO<sub>2</sub> capture and oxygen degradation experiments. The thermal degradation experiment uses this apparatus to load the TEA solution before it is placed into an autoclave reactor. See <a href="#sec2dot1-atmosphere-15-01479" class="html-sec">Section 2.1</a>, <a href="#sec2dot2-atmosphere-15-01479" class="html-sec">Section 2.2</a> and <a href="#sec2dot3-atmosphere-15-01479" class="html-sec">Section 2.3</a> for more information.</p>
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<p>Mean percentage CO<sub>2</sub> loading over time at 20 °C. CO<sub>2</sub> is sparged into TEA solution with/without 30 ppm NiNPs at concentrations of TEA (<b>a</b>) 3 wt%, (<b>b</b>) 5 wt%, (<b>c</b>) 7 wt%, (<b>d</b>) 10 wt%, (<b>e</b>), 15 wt%, (<b>f</b>), 20 wt%, and (<b>g</b>) 30 wt%. The horizontal dotted lines show the point at which there is the largest difference in CO<sub>2</sub> loading between the NiNPs and control samples; the time of this is shown with the right vertical dotted line and below in <a href="#atmosphere-15-01479-t001" class="html-table">Table 1</a>. The left vertical dotted line shows the time of the intercept with the NiNPs results line.</p>
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<p>Mean percentage CO<sub>2</sub> loading over time at 50 °C. CO<sub>2</sub> is sparged into TEA solution with/without 30 ppm NiNPs at concentrations of TEA (<b>a</b>) 3 wt%, (<b>b</b>) 5 wt%, (<b>c</b>) 7 wt%, (<b>d</b>) 10 wt%, (<b>e</b>), 15 wt%, (<b>f</b>), 20 wt%, and (<b>g</b>) 30 wt%. The horizontal dotted lines show the point at which there is the largest difference in CO<sub>2</sub> loading between the NiNPs and control samples; the time of this is shown with the right vertical dotted line and below in <a href="#atmosphere-15-01479-t003" class="html-table">Table 3</a>. The left vertical dotted line shows the time of the intercept with the NiNPs results line.</p>
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<p>Comparison of percentage enhancements of CO<sub>2</sub> absorption with NiNPs in TEA at 3–30 wt% concentrations and at 20 °C and 50 °C. See <a href="#app1-atmosphere-15-01479" class="html-app">Supplementary Materials Section S1</a> for the description of how enhancement is calculated.</p>
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<p>Photo of TEA (30 wt%) without and with NiNPs samples that are subjected to oxidative degradation.</p>
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<p>TEA % loss from day 0 due to oxidative degradation of TEA (30 wt%, 0.4 mole CO<sub>2</sub>/mole TEA, 55 °C, 0.35 L/min air, 7.5 mL/min CO<sub>2</sub>) without and with NiNPs over 7 days. The loss of TEA was calculated by the reduction in the size of the GC-MS TEA peak area compared to the TEA peak on day 0. Error bars show mean percentage error.</p>
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<p>Photo of TEA samples without and with NiNPs subjected to thermal degradation (the darker the color, the greater the degradation in the sample).</p>
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<p>TEA % loss from week 0 due to thermal degradation products in TEA (30 wt%, 0.5 mole CO<sub>2</sub>/mole TEA, 135 °C) without and with NiNPs over 5 weeks. The loss of TEA was calculated by the reduction in the size of the GC-MS TEA peak area compared to the TEA peak of day 0. Error bars show mean percentage error.</p>
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19 pages, 906 KiB  
Article
Forecasting of Local Lightning Using Spatial–Channel-Enhanced Recurrent Convolutional Neural Network
by Wei Zhou, Jinliang Li, Hongjie Wang, Donglai Zhang and Xupeng Wang
Atmosphere 2024, 15(12), 1478; https://doi.org/10.3390/atmos15121478 - 11 Dec 2024
Viewed by 349
Abstract
Lightning is a hazardous weather phenomenon, characterized by sudden occurrences and complex local distributions. It poses significant challenges for accurate forecasting, which is crucial for public safety and economic stability. Deep learning methods are often better than traditional numerical weather prediction (NWP) models [...] Read more.
Lightning is a hazardous weather phenomenon, characterized by sudden occurrences and complex local distributions. It poses significant challenges for accurate forecasting, which is crucial for public safety and economic stability. Deep learning methods are often better than traditional numerical weather prediction (NWP) models at capturing the spatiotemporal predictors of lightning events. However, these methods struggle to integrate predictors from diverse data sources, which leads to lower accuracy and interpretability. To address these challenges, the Multi-Scale Spatial–Channel-Enhanced Recurrent Convolutional Neural Network (SCE-RCNN) is proposed to improve forecasting accuracy and timeliness by utilizing multi-source data and enhanced attention mechanisms. The proposed model incorporates a multi-scale spatial–channel attention module and a cross-scale fusion module, which facilitates the integration of data from diverse sources. The multi-scale spatial–channel attention module utilizes a multi-scale convolutional network to extract spatial features at different spatial scales and employs a spatial–channel attention mechanism to focus on the most relevant regions for lightning prediction. Experimental results show that the SCE-RCNN model achieved a critical success index (CSI) of 0.83, a probability of detection (POD) of 0.991, and a false alarm rate (FAR) reduced to 0.351, outperforming conventional deep learning models across multiple prediction metrics. This research provides reliable lightning forecasts to support real-time decision-making, making significant contributions to aviation safety, outdoor event planning, and disaster risk management. The model’s high accuracy and low false alarm rate highlight its value in both academic research and practical applications. Full article
(This article belongs to the Special Issue The Challenge of Weather and Climate Prediction)
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<p>Model workflow diagram.</p>
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<p>The workflow of the multi-scale spatial–channel attention mechanism.</p>
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<p>Intra-scale joint attention module.</p>
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<p>Cross-scale cooperative fusion module.</p>
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<p>Predicted lightning for the next hour across regions and intensities.</p>
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<p>Critical success index (CSI) over time for different models.</p>
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<p>Performance metrics comparison among different model versions.</p>
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18 pages, 1492 KiB  
Article
Exposure to Extreme Temperatures and Change in Dietary Patterns in Korea
by Seungyeon Cho
Atmosphere 2024, 15(12), 1477; https://doi.org/10.3390/atmos15121477 - 11 Dec 2024
Viewed by 307
Abstract
Climate change has led to increased volatility in extreme temperatures, which poses a significant threat to human health. One way in which extreme temperatures impact health is through changes in dietary patterns, particularly food consumption and nutrient intake. This study uses a restricted-access [...] Read more.
Climate change has led to increased volatility in extreme temperatures, which poses a significant threat to human health. One way in which extreme temperatures impact health is through changes in dietary patterns, particularly food consumption and nutrient intake. This study uses a restricted-access version of 24 h dietary recall data from the 2018–2021 Korea National Health and Nutrition Examination Survey and meteorological data to examine the effect of heat and cold waves on food consumption and nutrient intake. The results suggest that cold waves increase individuals’ intake of key nutrients such as calories, protein, fat, saturated fat, and sodium. In contrast, heat waves have little to no significant effect on nutrient intake. Aside from the significant increase in the consumption of beer and chicken, the effects of heat or cold waves on overall food consumption are minimal. Depending on age and income level, cold and heat waves have different effects on food consumption and nutrient intake. This study suggests that temperature, particularly extreme heat and cold, plays a significant role in shaping individuals’ dietary patterns. Therefore, special attention is needed to maintain a balanced and healthy diet during extreme temperatures. Full article
(This article belongs to the Section Biometeorology and Bioclimatology)
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<p>Distribution of maximum temperature.</p>
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<p>Effects of temperatures on nutrient intake.</p>
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<p>Effects of temperatures on food consumption.</p>
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<p>Effects of temperatures on nutrient intake by age group.</p>
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<p>Effects of temperatures on food consumption by age group.</p>
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<p>Effects of temperatures on nutrient intake by income group.</p>
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<p>Effects of temperatures on food consumption by income group.</p>
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17 pages, 3410 KiB  
Article
The Aerosol Optical Depth Retrieval from Wide-Swath Imaging of DaQi-1 over Beijing
by Zhongting Wang, Ruijie Zhang, Ruizhi Chen and Hui Chen
Atmosphere 2024, 15(12), 1476; https://doi.org/10.3390/atmos15121476 - 10 Dec 2024
Viewed by 456
Abstract
The Wide-Swath Imaging (WSI) sensor is a Chinese satellite launched in 2022, capable of providing data at resolutions ranging from 75 to 600 m for monitoring aerosols, fire points, and dust, among other uses. In this study, we developed a Dark Dense Vegetation [...] Read more.
The Wide-Swath Imaging (WSI) sensor is a Chinese satellite launched in 2022, capable of providing data at resolutions ranging from 75 to 600 m for monitoring aerosols, fire points, and dust, among other uses. In this study, we developed a Dark Dense Vegetation method to retrieve the Aerosol Optical Depth (AOD) quickly from WSI 600 m data. First, after splitting into three types according to the Normalized Difference Vegetation Index (NDVI), we calculated the empirical parameters of land reflectance between the red (0.65 μm) and blue (0.47 μm) channels using Moderate Resolution Imaging Spectroradiometer (MODIS) reflectance products over the Beijing area. Second, the decrease in the NDVI was simulated and analyzed under different AODs and solar zenith angles, and we introduced an iterative inversion approach to account for it. The simulation retrievals demonstrated that the iterative inversion produced accurate results after less than four iterations. Thirdly, we utilized the atmospherically corrected NDVI for dark target identification and output the AOD result. Finally, retrieval experiments were conducted using WSI 600 m data collected over Beijing in 2023. The retrieved AOD images highlighted two air pollution events occurring during 3–8 March and 27–31 October 2023. The inversion results in 2023 showed a strong correlation with Aerosol Robotic Network station data (the correlation coefficient was greater than 0.9). Our method exhibited greater accuracy than the MODIS aerosol product, though it was less accurate than the Multi-Angle Implementation of Atmospheric Correction product. Full article
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<p>Filter response functions of WSI and MODIS in the channels which range from 380 nm to 900 nm.</p>
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<p>Flow chart of AOD retrieval method for WSI.</p>
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<p>The percentage histogram of pixel count over the Beijing area: (<b>a</b>) is surface reflectance in blue, green, red and NIR channels, and (<b>b</b>) is NDVI.</p>
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<p>The comparison of surface reflectance between red and blue: (<b>a</b>) is low vegetation, (<b>b</b>) is medium vegetation, (<b>c</b>) is high vegetation, and (<b>d</b>) is all of the vegetation. Dashed line represents the linear fitting line. The color represents the percentage of pixel numbers.</p>
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<p>The decreased NDVI under different AODs. The left is SZA = 21 degrees (<b>a</b>,<b>c</b>,<b>e</b>), while the right is SZA = 63 degrees (<b>b</b>,<b>d</b>,<b>f</b>). The top is low vegetation (<b>a</b>,<b>b</b>), the middle is medium vegetation (<b>c</b>,<b>d</b>), and the bottom is high vegetation (<b>e</b>,<b>f</b>).</p>
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<p>The maximum number of iterations changing with AOD and errors from measurements: (<b>a</b>) is low vegetation, (<b>b</b>) is medium vegetation, and (<b>c</b>) is high vegetation.</p>
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<p>Daily PM<sub>2.5</sub> concentration on 3–8 March 2023.</p>
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<p>WSI AOD images during a pollution event on 3–8 March 2023.</p>
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<p>Daily PM<sub>2.5</sub> concentration on 27–31 October 2023.</p>
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<p>WSI AOD images during a pollution event on 27–31 October 2023. (<b>a</b>) is October 27, (<b>b</b>) is October 28, (<b>c</b>) is October 29, (<b>d</b>) is October 30, and (<b>e</b>) is October 31.</p>
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<p>WSI AOD images during a pollution event on 27–31 October 2023. (<b>a</b>) is October 27, (<b>b</b>) is October 28, (<b>c</b>) is October 29, (<b>d</b>) is October 30, and (<b>e</b>) is October 31.</p>
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<p>AOD in 2023 over AERONET Beijing station. The yellow is AERONET, the green is WSI, the red is MYD04, and the black is MAIAC.</p>
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<p>AOD validation of WSI (<b>a</b>) MAIAC, (<b>b</b>) and MYD04, (<b>c</b>) with AERONET data. N represents the number of matched pixels. (<b>d</b>) All matched points, where the green is WSI, the red is MYD04, and the black is MAIAC.</p>
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<p>AOD validation of WSI (<b>a</b>) MAIAC, (<b>b</b>) and MYD04, (<b>c</b>) with AERONET data. N represents the number of matched pixels. (<b>d</b>) All matched points, where the green is WSI, the red is MYD04, and the black is MAIAC.</p>
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13 pages, 5759 KiB  
Article
Design and Performance Analysis of Meteorological Temperature Sensor Calibration Device Using Gas Cavities
by Yafei Huang, Chenhao Gao, Zhaopeng Wen, Fei Qian and Lijun He
Atmosphere 2024, 15(12), 1475; https://doi.org/10.3390/atmos15121475 - 10 Dec 2024
Viewed by 333
Abstract
In order to solve the problem of a meteorology temperature sensor not being able to touch a liquid, an open gas cavity structure immersed in the liquid was designed. According to the characteristics that the temperature sensing position of the meteorological temperature sensor [...] Read more.
In order to solve the problem of a meteorology temperature sensor not being able to touch a liquid, an open gas cavity structure immersed in the liquid was designed. According to the characteristics that the temperature sensing position of the meteorological temperature sensor is in the bottom area of the gas cavity, a simulation and experimental study of the bottom temperature field of φ50 mm cylindrical and φ(50-35-25) mm stepped column gas cavities were carried out. The experimental results at (−30~30) °C show that the gas stability of the gas cavities was better than that of the liquid constant temperature bath, and the performance of the cylindrical gas cavity was the best. The gas temperature stability of the stepped column gas cavity and the liquid constant temperature bath follow a strong trend. The maximum stability of the cylindrical gas cavity is 0.0054 °C, and the maximum stability of the stepped column gas cavity is 0.0080 °C. The results also show that the maximum uniformity of the stepped gas cavity is 0.0077 °C, and the maximum uniformity of the cylindrical gas cavity is 0.0528 °C. The uncertainty introduced in the measurement process was evaluated to ensure the confidence of the experimental data. The maximum value of the extended uncertainty was U = 0.0027 °C (k = 2). Compared with the solid-state constant temperature bath calibration method, the temperature sensor of different shapes can be directly placed into the gas cavity without the need for the meteorological temperature sensor to be closely attached to the wall of the gas cavity, and a sealing plug is used to seal the cavity mouth. The operation is very convenient, rapid turnover of the calibration of the meteorological temperature sensor can be achieved, and the work efficiency can be improved. Superior stability and uniformity can be obtained compared to gas constant temperature cavities. This study provides a valuable reference for the structural design of large-volume gas cavities and provides support and guarantee for global climate change monitoring. Full article
(This article belongs to the Section Atmospheric Techniques, Instruments, and Modeling)
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<p>Schematic diagram of meteorological temperature sensor calibration device using gas cavities.</p>
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<p>Structural design of gas cavities. (<b>a</b>) Cylindrical gas cavity; (<b>b</b>) stepped column gas cavity. Point A is the sensing position.</p>
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<p>Stability of gas cavities.</p>
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<p>The uniformity of point A’s circular section in each gas cavity at 2400 s. (<b>a</b>) −20 °C, cylindrical gas cavity; (<b>b</b>) −20 °C, stepped column gas cavity; (<b>c</b>) 0 °C, cylindrical gas cavity; (<b>d</b>) 0 °C, stepped column gas cavity; (<b>e</b>) 30 °C, cylindrical gas cavity; (<b>f</b>) 30 °C, stepped column gas cavity.</p>
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<p>Uniformity of gas cavities.</p>
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<p>Composition of meteorological temperature sensor calibration device using the gas cavities.</p>
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<p>Triple point water bottle calibration experiment.</p>
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<p>Calibration data of standard platinum resistance thermometer in the triple point water bottles. (<b>a</b>) DF2268; (<b>b</b>) DF2245.</p>
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<p>Stability of gas cavities.</p>
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13 pages, 4497 KiB  
Article
A Comparison of the Effects of Climate and Human Variability on the Thermal Resistance of Clothing
by Ferenc Ács, Zsófia Szalkai, Erzsébet Kristóf and Annamária Zsákai
Atmosphere 2024, 15(12), 1474; https://doi.org/10.3390/atmos15121474 - 10 Dec 2024
Viewed by 311
Abstract
We used a clothing thermal resistance model to investigate and compare the effects of climate and human variability on human thermal load. To investigate the effect of climate variability, we introduced the mean clothing thermal resistance rcl¯. For characterizing [...] Read more.
We used a clothing thermal resistance model to investigate and compare the effects of climate and human variability on human thermal load. To investigate the effect of climate variability, we introduced the mean clothing thermal resistance rcl¯. For characterizing the effect of human variability, we used the standard deviation of clothing thermal resistance rcl. We distinguished people based on their body type. We also defined the average human, a man and a woman, with thermal resistances of rcl,m and rcl,f. The investigation was carried out for the European region in the cold season for the period of 1981–2010. The climate variables were taken from the ERA5 reanalysis database. Our most important results are the following. (1) The macroscale pattern of the rcl¯ and rcl fields are very similar, based on which it can be stated that human variability does not modify the spatial distribution of rcl¯. (2) The rcl values are roughly a quarter of the rcl¯ values. The highest rcl¯ values (3.2–3.4 clo) are in Lapland, and the smallest (1–1.2 clo) in Andalusia. (3) The macroscale pattern of the rcl,m and rcl,f fields is similar to the macroscale pattern of the rcl values of the mesomorphic person rcl,2. The field of rcl,2 can be used for climate classification purposes. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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<p>The European region (25° W–50° E/35° N–72.5° N longitude/latitude lines) studied together with elevation level notifications. The red lines denote 68° N, 47° N, and 37° N latitude lines.</p>
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<p>The <span class="html-italic">M-BMI</span> point cloud for walking men (blue) and women (red). The three black notations represent an ectomorphic woman, a mesomorphic man, and an endomorphic woman whose anthropometric data are used in the study. Sources of the data: [<a href="#B27-atmosphere-15-01474" class="html-bibr">27</a>,<a href="#B28-atmosphere-15-01474" class="html-bibr">28</a>,<a href="#B29-atmosphere-15-01474" class="html-bibr">29</a>].</p>
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<p>Spatial distribution of mean <span class="html-italic">r<sub>cl</sub></span> values in the European region for the cold season in the period of 1981–2010. <math display="inline"><semantics> <mrow> <mover accent="true"> <mrow> <msub> <mrow> <mi>r</mi> </mrow> <mrow> <mi>c</mi> <mi>l</mi> </mrow> </msub> </mrow> <mo>¯</mo> </mover> <mtext> </mtext> </mrow> </semantics></math>values were obtained by averaging the <span class="html-italic">r<sub>cl</sub></span> values of people with ectomorphic, mesomorphic, and endomorphic body types. The walking speed of people is 1.1 m s<sup>−1</sup>.</p>
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<p>The European region’s climate in the period of 1971–2000 according to Feddema [<a href="#B26-atmosphere-15-01474" class="html-bibr">26</a>].</p>
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<p>Spatial distribution of the standard deviation of clothing thermal resistance values in the European region for the cold season in the period of 1981–2010. <math display="inline"><semantics> <mrow> <mo>∆</mo> <msub> <mrow> <mi>r</mi> </mrow> <mrow> <mi>c</mi> <mi>l</mi> </mrow> </msub> </mrow> </semantics></math> values were obtained by averaging the r<sub>cl</sub> values of people with ectomorphic, mesomorphic, and endomorphic body types. The walking speed of people is 1.1 m s<sup>−1</sup>.</p>
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<p>Spatial distribution of clothing thermal resistance values for the average man in the European region for the cold season in the period of 1981–2010. The average man is walking at a speed of 1.1 m s<sup>−1</sup>.</p>
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<p>Spatial distribution of clothing thermal resistance values for the average woman in the European region for the cold season in the period of 1981–2010. The average woman is walking at a speed of 1.1 m s<sup>−1</sup>.</p>
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<p>Spatial distribution of clothing thermal resistance values for a mesomorphic person in the European region in the period 1981–2010. The mesomorphic person is walking at a speed of 1.1 m s<sup>−1</sup>.</p>
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19 pages, 8828 KiB  
Article
Construction of Heavy-Duty Diesel Vehicle Atmospheric Pollutant Emission Inventory Based on Onboard Diagnosis Data
by Ting Chen, Yangxin Xiong, Weidong Zhao, Bo Lin, Zehuang He, Feiyang Tao and Xiang Hu
Atmosphere 2024, 15(12), 1473; https://doi.org/10.3390/atmos15121473 - 10 Dec 2024
Viewed by 392
Abstract
Motor vehicles emit a large amount of air pollutants. NOx and particulate matter (PM) account for 53.2% and 74.7%, respectively, of vehicle emissions in China. Using the technical guidelines for compiling road vehicle emission inventories, the emission factors based on the onboard diagnostics [...] Read more.
Motor vehicles emit a large amount of air pollutants. NOx and particulate matter (PM) account for 53.2% and 74.7%, respectively, of vehicle emissions in China. Using the technical guidelines for compiling road vehicle emission inventories, the emission factors based on the onboard diagnostics (OBD) system of heavy-duty diesel vehicles are obtained. The trajectory of heavy-duty diesel vehicles is corrected using big data interpolation, and the correction coefficients for different vehicle speeds are fitted to calculate the corresponding correction factors. Simultaneously, the Weather Research and Forecasting model is used for the meteorological correction of emissions, a heavy-duty diesel vehicle emission inventory under the community multiscale air quality model is established, and the distribution characteristics of pollution emissions from heavy-duty diesel vehicles in Chengdu are analyzed at the time and space levels. Overall, the pollutant gasses emitted by heavy-duty diesel vehicles in Chengdu are largely concentrated at the city center. In 2023, the total annual emissions of the pollutants NOx, CO, fine PM, and volatile organic compounds from heavy-duty diesel vehicles in Chengdu were 10,590.60, 28,852.90, 686.18, and 657.60 tons, respectively. NOx and CO have the highest proportions among the major pollutants, accounting for 70.7% and 26%, respectively. Full article
(This article belongs to the Section Air Quality)
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<p>Overview of the research area.</p>
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<p>Scatter distribution of vehicle speed (x) and GPS instantaneous vehicle speed (y).</p>
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<p>OBD data of GFX and RAW (<b>a</b>) and LINE and RAW (<b>b</b>) (the blue dots in the figure represent the original trajectory points of the OBD data, while the red dots represent the corrected trajectory points, which overlap when directly read).</p>
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<p>Daily variation in pollutant emissions under different interpolation methods.(<b>a</b>) NO<sub>x</sub>, (<b>b</b>) CO, (<b>c</b>) PM<sub>2.5</sub>, (<b>d</b>) VOC<sub>S</sub>.</p>
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<p>Diurnal variation in pollutant emissions under different interpolation methods.</p>
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<p>Diurnal variation in pollutant emissions under different interpolation methods.</p>
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<p>Hourly variation in pollutant emissions under GFX method.</p>
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<p>Spatial distribution of CO, NOx, PM<sub>2.5</sub>, and VOC<sub>S</sub> emissions calculated by RAW.</p>
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<p>Spatial distribution of CO, NOx, PM<sub>2.5</sub>, and VOC<sub>S</sub> emissions calculated by LINE.</p>
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<p>Spatial distribution of CO, NOx, PM<sub>2.5</sub>, and VOC<sub>S</sub> emissions calculated by GFX.</p>
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<p>Total pollutant emissions from various districts and counties in Chengdu City.</p>
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13 pages, 5244 KiB  
Article
Impact of Nitrogen Dioxide (NO2) Pollution on Asthma: The Case of Louisiana State (2005–2020)
by Keshav Bhattarai, Lok Lamsal, Madhu Gyawali, Sujan Neupane, Shiva P. Gautam, Arundhati Bakshi and John Yeager
Atmosphere 2024, 15(12), 1472; https://doi.org/10.3390/atmos15121472 - 10 Dec 2024
Viewed by 553
Abstract
This study explores the connection between tropospheric nitrogen dioxide (NO2) vertical column density levels and asthma hospitalization cases in Louisiana from 2005 to 2020. Utilizing NO2 data from NASA’s Ozone Measurement Instrument (OMI) aboard the Aura satellite, the research integrates [...] Read more.
This study explores the connection between tropospheric nitrogen dioxide (NO2) vertical column density levels and asthma hospitalization cases in Louisiana from 2005 to 2020. Utilizing NO2 data from NASA’s Ozone Measurement Instrument (OMI) aboard the Aura satellite, the research integrates these atmospheric measurements with socioeconomic data at the census tract level. This study employs a generalized linear mixed model (GLIMMIX) with a logit link and Beta distribution to analyze the relationship between seasonal NO2 levels and asthma hospitalization cases during winter, fall, spring, and summer. By analyzing OMI data, this research quantifies seasonal variations in NO2 levels and their corresponding impact on asthma hospitalizations. The findings reveal a relationship between NO2 levels and asthma hospitalizations, particularly in communities with high Black and/or low-income populations, with the strongest effects observed during winter. Specifically, the analysis shows that, for each unit increase in NO2 levels, the odds of asthma-related hospitalizations increase by approximately 26.3% (p < 0.0001), with a 95% confidence interval ranging from 23.3% to 29.5%. Assuming a causal link between NO2 and asthma, these findings suggest that reducing NO2 emissions could alleviate healthcare burdens associated with respiratory diseases such as asthma. Full article
(This article belongs to the Special Issue Remote Sensing and In Situ Measurements of Aerosols and Trace Gases)
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<p>Overview of demographic, socioeconomic, environmental, and health metrics by census tract (Louisiana; 2005–2020). (<b>a</b>) Average annual population (2005–2020). (<b>b</b>) Average annual White; and (<b>c</b>) Black population (2005–2020). (<b>d</b>) Average income (2005–2020). (<b>e</b>) Major roads, power plants, petroleum refineries, and natural gas processing plants. (<b>f</b>) Percentage of Asthma hospitalizations (average from 2005 to 2020).</p>
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<p>Seasonal distribution of tropospheric NO<sub>2</sub> columns over Louisiana, illustrating higher concentrations in urban and industrial areas, particularly during winter and fall, with spatial patterns resolved at a census tract scale in the lower row.</p>
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<p>Seasonal variation in tropospheric NO<sub>2</sub> column concentrations (10<sup>15</sup> molec cm⁻<sup>2</sup>) within and outside Louisiana’s petrochemical corridor from 2005 to 2020. The black bars depict NO<sub>2</sub> levels within the petrochemical corridor, while the dotted red line represents levels outside the corridor. The bar graphs are organized by season: Winter (December, January, February), Spring (March, April, May), Summer (June, July, August), and Fall (September, October, November), for each year within the study period. The dotted red line consistently parallels the black bars, reflecting lower NO<sub>2</sub> concentrations outside the corridor.</p>
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<p>Spatial analysis of tropospheric NO<sub>2</sub> column (10<sup>15</sup> molec cm<sup>−2</sup>) with demographic and socioeconomic characteristics (Louisiana; 2005–2020). (<b>a</b>) Level of tropospheric NO<sub>2</sub> column. (<b>b</b>) Distribution of the Black population. (<b>c</b>) Distribution of White population. (<b>d</b>) Distribution of income level. (<b>e</b>) Occurrence of asthma hospitalization cases.</p>
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