CS204038B2 - Granulated organosilane preparation - Google Patents
Granulated organosilane preparation Download PDFInfo
- Publication number
- CS204038B2 CS204038B2 CS786841A CS684178A CS204038B2 CS 204038 B2 CS204038 B2 CS 204038B2 CS 786841 A CS786841 A CS 786841A CS 684178 A CS684178 A CS 684178A CS 204038 B2 CS204038 B2 CS 204038B2
- Authority
- CS
- Czechoslovakia
- Prior art keywords
- weight
- organosilane
- preparation
- carbon atoms
- organosilanes
- Prior art date
Links
- 238000002360 preparation method Methods 0.000 title claims abstract description 47
- 150000001282 organosilanes Chemical class 0.000 title claims abstract description 43
- 239000006229 carbon black Substances 0.000 claims abstract description 24
- 125000004432 carbon atom Chemical group C* 0.000 claims abstract description 15
- 125000000217 alkyl group Chemical group 0.000 claims abstract description 5
- DOIRQSBPFJWKBE-UHFFFAOYSA-N dibutyl phthalate Chemical compound CCCCOC(=O)C1=CC=CC=C1C(=O)OCCCC DOIRQSBPFJWKBE-UHFFFAOYSA-N 0.000 claims description 10
- 239000011164 primary particle Substances 0.000 claims description 9
- 238000010521 absorption reaction Methods 0.000 claims description 5
- -1 alkyl radical Chemical class 0.000 claims description 5
- 241000872198 Serjania polyphylla Species 0.000 claims description 4
- 239000008187 granular material Substances 0.000 abstract description 8
- 125000003545 alkoxy group Chemical group 0.000 abstract description 3
- 125000002947 alkylene group Chemical group 0.000 abstract description 2
- 239000000203 mixture Substances 0.000 description 31
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 description 19
- 235000019241 carbon black Nutrition 0.000 description 19
- 229920001971 elastomer Polymers 0.000 description 15
- 239000005060 rubber Substances 0.000 description 15
- 229910000077 silane Inorganic materials 0.000 description 14
- BLRPTPMANUNPDV-UHFFFAOYSA-N Silane Chemical compound [SiH4] BLRPTPMANUNPDV-UHFFFAOYSA-N 0.000 description 13
- 238000003860 storage Methods 0.000 description 12
- 238000004132 cross linking Methods 0.000 description 11
- 239000000945 filler Substances 0.000 description 9
- VYPSYNLAJGMNEJ-UHFFFAOYSA-N Silicium dioxide Chemical compound O=[Si]=O VYPSYNLAJGMNEJ-UHFFFAOYSA-N 0.000 description 8
- 239000007788 liquid Substances 0.000 description 7
- 239000000843 powder Substances 0.000 description 6
- BPQQTUXANYXVAA-UHFFFAOYSA-N Orthosilicate Chemical compound [O-][Si]([O-])([O-])[O-] BPQQTUXANYXVAA-UHFFFAOYSA-N 0.000 description 4
- NINIDFKCEFEMDL-UHFFFAOYSA-N Sulfur Chemical compound [S] NINIDFKCEFEMDL-UHFFFAOYSA-N 0.000 description 4
- 230000007062 hydrolysis Effects 0.000 description 4
- 238000006460 hydrolysis reaction Methods 0.000 description 4
- 235000012239 silicon dioxide Nutrition 0.000 description 4
- 229920003048 styrene butadiene rubber Polymers 0.000 description 4
- VTHOKNTVYKTUPI-UHFFFAOYSA-N triethoxy-[3-(3-triethoxysilylpropyltetrasulfanyl)propyl]silane Chemical compound CCO[Si](OCC)(OCC)CCCSSSSCCC[Si](OCC)(OCC)OCC VTHOKNTVYKTUPI-UHFFFAOYSA-N 0.000 description 4
- 238000006243 chemical reaction Methods 0.000 description 3
- 239000000428 dust Substances 0.000 description 3
- 238000004519 manufacturing process Methods 0.000 description 3
- 238000000034 method Methods 0.000 description 3
- 125000000956 methoxy group Chemical group [H]C([H])([H])O* 0.000 description 3
- GRVDJDISBSALJP-UHFFFAOYSA-N methyloxidanyl Chemical compound [O]C GRVDJDISBSALJP-UHFFFAOYSA-N 0.000 description 3
- 239000002245 particle Substances 0.000 description 3
- 239000011049 pearl Substances 0.000 description 3
- 239000012744 reinforcing agent Substances 0.000 description 3
- RMAQACBXLXPBSY-UHFFFAOYSA-N silicic acid Chemical compound O[Si](O)(O)O RMAQACBXLXPBSY-UHFFFAOYSA-N 0.000 description 3
- 239000006238 High Abrasion Furnace Substances 0.000 description 2
- 239000002174 Styrene-butadiene Substances 0.000 description 2
- 238000005299 abrasion Methods 0.000 description 2
- 239000011324 bead Substances 0.000 description 2
- 238000010410 dusting Methods 0.000 description 2
- 238000009472 formulation Methods 0.000 description 2
- 230000002035 prolonged effect Effects 0.000 description 2
- 150000004756 silanes Chemical class 0.000 description 2
- 239000000377 silicon dioxide Substances 0.000 description 2
- 239000000126 substance Substances 0.000 description 2
- 238000012360 testing method Methods 0.000 description 2
- 238000004073 vulcanization Methods 0.000 description 2
- 239000005995 Aluminium silicate Substances 0.000 description 1
- LFQSCWFLJHTTHZ-UHFFFAOYSA-N Ethanol Chemical compound CCO LFQSCWFLJHTTHZ-UHFFFAOYSA-N 0.000 description 1
- 239000005909 Kieselgur Substances 0.000 description 1
- XUIMIQQOPSSXEZ-UHFFFAOYSA-N Silicon Chemical group [Si] XUIMIQQOPSSXEZ-UHFFFAOYSA-N 0.000 description 1
- 239000013543 active substance Substances 0.000 description 1
- 239000002318 adhesion promoter Substances 0.000 description 1
- 235000012211 aluminium silicate Nutrition 0.000 description 1
- 125000004429 atom Chemical group 0.000 description 1
- 150000004649 carbonic acid derivatives Chemical class 0.000 description 1
- 239000004927 clay Substances 0.000 description 1
- 238000003776 cleavage reaction Methods 0.000 description 1
- 230000000052 comparative effect Effects 0.000 description 1
- 238000011109 contamination Methods 0.000 description 1
- 230000008021 deposition Effects 0.000 description 1
- 230000006866 deterioration Effects 0.000 description 1
- 238000010348 incorporation Methods 0.000 description 1
- 238000011534 incubation Methods 0.000 description 1
- NLYAJNPCOHFWQQ-UHFFFAOYSA-N kaolin Chemical compound O.O.O=[Al]O[Si](=O)O[Si](=O)O[Al]=O NLYAJNPCOHFWQQ-UHFFFAOYSA-N 0.000 description 1
- 239000000463 material Substances 0.000 description 1
- 238000005259 measurement Methods 0.000 description 1
- 239000010445 mica Substances 0.000 description 1
- 229910052618 mica group Inorganic materials 0.000 description 1
- STSDHUBQQWBRBH-UHFFFAOYSA-N n-cyclohexyl-1,3-benzothiazole-2-sulfonamide Chemical compound N=1C2=CC=CC=C2SC=1S(=O)(=O)NC1CCCCC1 STSDHUBQQWBRBH-UHFFFAOYSA-N 0.000 description 1
- QIQXTHQIDYTFRH-UHFFFAOYSA-N octadecanoic acid Chemical group CCCCCCCCCCCCCCCCCC(O)=O QIQXTHQIDYTFRH-UHFFFAOYSA-N 0.000 description 1
- 150000003961 organosilicon compounds Chemical class 0.000 description 1
- 239000004033 plastic Substances 0.000 description 1
- 229920003023 plastic Polymers 0.000 description 1
- 229920001296 polysiloxane Polymers 0.000 description 1
- 230000002250 progressing effect Effects 0.000 description 1
- 125000001436 propyl group Chemical group [H]C([*])([H])C([H])([H])C([H])([H])[H] 0.000 description 1
- 239000010453 quartz Substances 0.000 description 1
- 230000035484 reaction time Effects 0.000 description 1
- 230000003014 reinforcing effect Effects 0.000 description 1
- 238000010057 rubber processing Methods 0.000 description 1
- 238000013040 rubber vulcanization Methods 0.000 description 1
- 230000007017 scission Effects 0.000 description 1
- 229910052710 silicon Inorganic materials 0.000 description 1
- 239000007787 solid Substances 0.000 description 1
- 239000004071 soot Substances 0.000 description 1
- 238000013112 stability test Methods 0.000 description 1
- 239000007858 starting material Substances 0.000 description 1
- 229940124530 sulfonamide Drugs 0.000 description 1
- 150000003456 sulfonamides Chemical class 0.000 description 1
- 229910052717 sulfur Inorganic materials 0.000 description 1
- 239000011593 sulfur Substances 0.000 description 1
- 125000004434 sulfur atom Chemical group 0.000 description 1
- XLYOFNOQVPJJNP-UHFFFAOYSA-N water Substances O XLYOFNOQVPJJNP-UHFFFAOYSA-N 0.000 description 1
- 238000005303 weighing Methods 0.000 description 1
- RNWHGQJWIACOKP-UHFFFAOYSA-N zinc;oxygen(2-) Chemical group [O-2].[Zn+2] RNWHGQJWIACOKP-UHFFFAOYSA-N 0.000 description 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K3/00—Use of inorganic substances as compounding ingredients
- C08K3/02—Elements
- C08K3/04—Carbon
-
- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07F—ACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
- C07F7/00—Compounds containing elements of Groups 4 or 14 of the Periodic Table
- C07F7/02—Silicon compounds
- C07F7/08—Compounds having one or more C—Si linkages
- C07F7/18—Compounds having one or more C—Si linkages as well as one or more C—O—Si linkages
- C07F7/1804—Compounds having Si-O-C linkages
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J3/00—Processes of treating or compounding macromolecular substances
- C08J3/20—Compounding polymers with additives, e.g. colouring
- C08J3/22—Compounding polymers with additives, e.g. colouring using masterbatch techniques
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/54—Silicon-containing compounds
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/54—Silicon-containing compounds
- C08K5/548—Silicon-containing compounds containing sulfur
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J2321/00—Characterised by the use of unspecified rubbers
Landscapes
- Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Health & Medical Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Compositions Of Macromolecular Compounds (AREA)
- Pigments, Carbon Blacks, Or Wood Stains (AREA)
- Silicon Polymers (AREA)
Applications Claiming Priority (1)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
DE2747277A DE2747277C2 (de) | 1977-10-21 | 1977-10-21 | Granulatförmige Organosilan-Präparation, deren Herstellung und Verwendung |
Publications (1)
Publication Number | Publication Date |
---|---|
CS204038B2 true CS204038B2 (en) | 1981-03-31 |
Family
ID=6021934
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
CS786841A CS204038B2 (en) | 1977-10-21 | 1978-10-20 | Granulated organosilane preparation |
Country Status (16)
Country | Link |
---|---|
US (1) | US4128438A (ja) |
JP (1) | JPS5468860A (ja) |
AU (1) | AU512265B2 (ja) |
BE (1) | BE862381A (ja) |
BR (1) | BR7801477A (ja) |
CA (1) | CA1099855A (ja) |
CS (1) | CS204038B2 (ja) |
DD (1) | DD133961A5 (ja) |
DE (1) | DE2747277C2 (ja) |
FR (1) | FR2406651A1 (ja) |
GB (1) | GB1588060A (ja) |
IT (1) | IT1155825B (ja) |
MY (1) | MY8500419A (ja) |
NL (1) | NL186254C (ja) |
SG (1) | SG5084G (ja) |
SU (1) | SU795495A3 (ja) |
Families Citing this family (41)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
DE2933346C2 (de) * | 1979-08-17 | 1982-07-01 | Degussa Ag, 6000 Frankfurt | Silan/Füllstoff-Präparationen, Verfahren zu deren Herstellung und Anwendung derselben |
DE3305373C2 (de) * | 1983-02-17 | 1985-07-11 | Degussa Ag, 6000 Frankfurt | Elastische Formmasse, Verfahren zum Herstellen und Verformen und Verwendung derselben |
JPS59189933A (ja) * | 1983-04-11 | 1984-10-27 | Shin Etsu Chem Co Ltd | 自己乳化性シリコーン消泡剤組成物 |
DE3314742C2 (de) * | 1983-04-23 | 1987-04-02 | Degussa Ag, 6000 Frankfurt | Verfahren zur Herstellung von an der Oberfläche modifizierten natürlichen, oxidischen oder silikatischen Füllstoffen und deren Verwendung |
JPS6248743A (ja) * | 1985-08-28 | 1987-03-03 | Shin Etsu Chem Co Ltd | ゴム組成物 |
DE4023537A1 (de) * | 1990-07-25 | 1992-01-30 | Degussa | Mit organosiliciumverbindungen chemisch modifizierte russe, verfahren zu deren herstellung und deren verwendung |
DE4119959A1 (de) * | 1991-06-18 | 1992-12-24 | Degussa | Verfahren zur herstellung von vulkanisierbaren, mit russ gefuellten kunststoff- und kautschukmischungen |
IT1256263B (it) * | 1992-12-30 | 1995-11-29 | Bayer Italia Spa | Granulati di coloranti scorrevoli,chimicamente resistenti,loro preparazione e loro impiego |
US5653875A (en) * | 1994-02-04 | 1997-08-05 | Supelco, Inc. | Nucleophilic bodies bonded to siloxane and use thereof for separations from sample matrices |
US5494955A (en) * | 1994-04-08 | 1996-02-27 | Columbian Chemicals Company | Use of silane coupling agent with carbon black to enhance the balance of reinforcement properties of rubber compounds |
DE4435311A1 (de) * | 1994-10-01 | 1996-04-04 | Huels Silicone Gmbh | Verstärkungsadditive |
DE19529916A1 (de) * | 1995-08-16 | 1997-02-20 | Bayer Ag | Verfahren zur Herstellung von immobilisierten polysulfidischen Silanen und deren Verwendung zur Herstellung von Kautschukmischungen und -vulkanisaten |
US6005027A (en) * | 1995-08-16 | 1999-12-21 | Witco Corporation | Stable silane compositions on silica carrier |
DE19732725A1 (de) * | 1997-07-30 | 1999-02-04 | Degussa | Mischungen, bestehend aus Bis(silylorganyl)polysulfanen und Silylorganylthiocyanaten, ihre Herstellung und Verwendung |
US6147147A (en) * | 1998-05-08 | 2000-11-14 | Flow Polymers, Inc. | Coupling agent composition |
DE19955850A1 (de) | 1999-11-20 | 2001-06-07 | Degussa | Granulatförmige Organosilan-Präparation, Verfahren zu ihrer Herstellung und ihre Verwendung |
CA2316127C (en) | 1999-12-13 | 2009-01-06 | The Goodyear Tire & Rubber Company | Hose construction having inner core of hydrogenated nbr |
US6211345B1 (en) | 1999-12-22 | 2001-04-03 | Witco Corporation | Synthesis of cyclic sulfur silanes |
US6567836B1 (en) | 1999-12-23 | 2003-05-20 | Intel Corporation | Multi-level carry-skip adder |
US6358305B1 (en) | 2000-03-08 | 2002-03-19 | Isp Investments Inc. | Darkened headlap manufacturing process and product produced thereby |
US6359046B1 (en) | 2000-09-08 | 2002-03-19 | Crompton Corporation | Hydrocarbon core polysulfide silane coupling agents for filled elastomer compositions |
DE10216657A1 (de) * | 2002-04-15 | 2003-10-23 | Rhein Chemie Rheinau Gmbh | Vulkanisierbare Kautschukmischungen und Verfahren zur Herstellung |
ES2268210T5 (es) * | 2003-05-02 | 2010-05-19 | Evonik Degussa Gmbh | Mezcla madre de organosilano. |
EP1714999B1 (en) * | 2004-02-10 | 2011-08-24 | The Yokohama Rubber Co., Ltd. | Rubber composition for pneumatic tire |
US7820751B2 (en) * | 2004-02-10 | 2010-10-26 | The Yokohama Rubber Co., Ltd. | Rubber composition for pneumatic tire |
RU2358991C2 (ru) | 2004-09-01 | 2009-06-20 | Сираиси Когио Кайся, Лтд. | Порошкообразная белая композиция промотора вулканизации и композиции каучука |
US7833339B2 (en) | 2006-04-18 | 2010-11-16 | Franklin Industrial Minerals | Mineral filler composition |
JP4499658B2 (ja) | 2005-12-26 | 2010-07-07 | 住友ゴム工業株式会社 | ゴム組成物およびそれを用いた空気入りタイヤ |
US7696269B2 (en) | 2006-12-28 | 2010-04-13 | Momentive Performance Materials Inc. | Silated core polysulfides, their preparation and use in filled elastomer compositions |
US7968636B2 (en) | 2006-12-28 | 2011-06-28 | Continental Ag | Tire compositions and components containing silated cyclic core polysulfides |
US7687558B2 (en) | 2006-12-28 | 2010-03-30 | Momentive Performance Materials Inc. | Silated cyclic core polysulfides, their preparation and use in filled elastomer compositions |
US7737202B2 (en) | 2006-12-28 | 2010-06-15 | Momentive Performance Materials Inc. | Free-flowing filler composition and rubber composition containing same |
US7968633B2 (en) | 2006-12-28 | 2011-06-28 | Continental Ag | Tire compositions and components containing free-flowing filler compositions |
US8592506B2 (en) | 2006-12-28 | 2013-11-26 | Continental Ag | Tire compositions and components containing blocked mercaptosilane coupling agent |
US7968635B2 (en) | 2006-12-28 | 2011-06-28 | Continental Ag | Tire compositions and components containing free-flowing filler compositions |
US7968634B2 (en) | 2006-12-28 | 2011-06-28 | Continental Ag | Tire compositions and components containing silated core polysulfides |
US7960460B2 (en) | 2006-12-28 | 2011-06-14 | Momentive Performance Materials, Inc. | Free-flowing filler composition and rubber composition containing same |
US7781606B2 (en) | 2006-12-28 | 2010-08-24 | Momentive Performance Materials Inc. | Blocked mercaptosilane coupling agents, process for making and uses in rubber |
US20120090720A1 (en) | 2010-10-19 | 2012-04-19 | Veyance Technologies, Inc. | Fluid resistant high temperature hose |
US20140296375A1 (en) | 2011-10-24 | 2014-10-02 | Bridgestone Americas Tire Operations, Llc | Silica-Filled Rubber Composition And Method For Making The Same |
DE102012108096A1 (de) * | 2012-08-31 | 2014-03-06 | Continental Reifen Deutschland Gmbh | Verfahren zur Regenerierung von schwefelvernetzten Gummivulkanisaten zu Regeneraten |
Family Cites Families (7)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
FR1459019A (fr) * | 1965-08-09 | 1966-04-29 | Fr Des Silicates Speciaux Sifr | Pigments modifiés en surface |
US3415775A (en) * | 1966-03-29 | 1968-12-10 | Monsanto Co | Blends of n-alkyl-n'-aryl phenylene diamines and a carrier |
US3873489A (en) * | 1971-08-17 | 1975-03-25 | Degussa | Rubber compositions containing silica and an organosilane |
DE2144378B2 (de) * | 1971-09-04 | 1975-08-07 | Bayer Ag, 5090 Leverkusen | Verfahren zur Agglomeration von Kautschukchemikalien |
US4005170A (en) * | 1973-09-14 | 1977-01-25 | Cabot Corporation | Preparation of pelletized carbon blacks |
AT332642B (de) * | 1973-10-11 | 1976-10-11 | Degussa | Vulkanisierbare kautschukmischungen fur reifen-laufflachen und vormischung hiefur |
DE2536674C3 (de) * | 1975-08-18 | 1979-09-27 | Deutsche Gold- Und Silber-Scheideanstalt Vormals Roessler, 6000 Frankfurt | Vernetzbare Mischungen auf Basis von Kautschuk, Organosilanen und silikatischen Füllstoffen |
-
1977
- 1977-10-21 DE DE2747277A patent/DE2747277C2/de not_active Expired
- 1977-12-21 GB GB53156/77A patent/GB1588060A/en not_active Expired
- 1977-12-23 DD DD77202927A patent/DD133961A5/xx unknown
- 1977-12-27 BE BE6046291A patent/BE862381A/xx not_active IP Right Cessation
-
1978
- 1978-01-05 SU SU782562403A patent/SU795495A3/ru active
- 1978-01-06 AU AU32225/78A patent/AU512265B2/en not_active Expired
- 1978-01-25 JP JP713978A patent/JPS5468860A/ja active Granted
- 1978-01-30 CA CA295,934A patent/CA1099855A/en not_active Expired
- 1978-01-31 US US05/873,967 patent/US4128438A/en not_active Expired - Lifetime
- 1978-02-13 FR FR7804007A patent/FR2406651A1/fr active Granted
- 1978-02-15 IT IT48056/78A patent/IT1155825B/it active
- 1978-03-10 BR BR7801477A patent/BR7801477A/pt unknown
- 1978-03-23 NL NLAANVRAGE7803190,A patent/NL186254C/xx not_active IP Right Cessation
- 1978-10-20 CS CS786841A patent/CS204038B2/cs unknown
-
1984
- 1984-01-18 SG SG50/84A patent/SG5084G/en unknown
-
1985
- 1985-12-30 MY MY419/85A patent/MY8500419A/xx unknown
Also Published As
Publication number | Publication date |
---|---|
DE2747277A1 (de) | 1979-04-26 |
IT7848056A0 (it) | 1978-02-15 |
IT1155825B (it) | 1987-01-28 |
GB1588060A (en) | 1981-04-15 |
SU795495A3 (ru) | 1981-01-07 |
AU3222578A (en) | 1979-07-12 |
NL186254B (nl) | 1990-05-16 |
DD133961A5 (de) | 1979-01-31 |
DE2747277C2 (de) | 1982-06-09 |
AU512265B2 (en) | 1980-10-02 |
FR2406651B1 (ja) | 1981-05-29 |
NL186254C (nl) | 1990-10-16 |
JPS5468860A (en) | 1979-06-02 |
US4128438A (en) | 1978-12-05 |
NL7803190A (nl) | 1979-04-24 |
BR7801477A (pt) | 1979-05-22 |
JPS6131137B2 (ja) | 1986-07-18 |
SG5084G (en) | 1985-02-01 |
BE862381A (fr) | 1978-06-27 |
MY8500419A (en) | 1985-12-31 |
CA1099855A (en) | 1981-04-28 |
FR2406651A1 (fr) | 1979-05-18 |
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