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WO2008123311A1 - 二次電池用正極材料の製造方法 - Google Patents

二次電池用正極材料の製造方法 Download PDF

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Publication number
WO2008123311A1
WO2008123311A1 PCT/JP2008/055749 JP2008055749W WO2008123311A1 WO 2008123311 A1 WO2008123311 A1 WO 2008123311A1 JP 2008055749 W JP2008055749 W JP 2008055749W WO 2008123311 A1 WO2008123311 A1 WO 2008123311A1
Authority
WO
WIPO (PCT)
Prior art keywords
transition metal
lithium
positive electrode
electrode material
secondary battery
Prior art date
Application number
PCT/JP2008/055749
Other languages
English (en)
French (fr)
Inventor
Atsuo Yamada
Shogo Hayase
Yoshiki Fujita
Shinichi Nishimura
Mamoru Tachikawa
Takakazu Hino
Original Assignee
Tokyo Institute Of Technology
Dow Corning Toray Co., Ltd.
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Tokyo Institute Of Technology, Dow Corning Toray Co., Ltd. filed Critical Tokyo Institute Of Technology
Priority to US12/532,956 priority Critical patent/US8349217B2/en
Priority to EP08738937A priority patent/EP2166600A4/en
Priority to JP2009509146A priority patent/JPWO2008123311A1/ja
Publication of WO2008123311A1 publication Critical patent/WO2008123311A1/ja

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    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/58—Selection of substances as active materials, active masses, active liquids of inorganic compounds other than oxides or hydroxides, e.g. sulfides, selenides, tellurides, halogenides or LiCoFy; of polyanionic structures, e.g. phosphates, silicates or borates
    • H01M4/5825—Oxygenated metallic salts or polyanionic structures, e.g. borates, phosphates, silicates, olivines
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/04—Processes of manufacture in general
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/50—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of manganese
    • H01M4/505—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of manganese of mixed oxides or hydroxides containing manganese for inserting or intercalating light metals, e.g. LiMn2O4 or LiMn2OxFy
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/48—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides
    • H01M4/52—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of nickel, cobalt or iron
    • H01M4/525—Selection of substances as active materials, active masses, active liquids of inorganic oxides or hydroxides of nickel, cobalt or iron of mixed oxides or hydroxides containing iron, cobalt or nickel for inserting or intercalating light metals, e.g. LiNiO2, LiCoO2 or LiCoOxFy
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/052—Li-accumulators
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/058—Construction or manufacture
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/136—Electrodes based on inorganic compounds other than oxides or hydroxides, e.g. sulfides, selenides, tellurides, halogenides or LiCoFy
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/139—Processes of manufacture
    • H01M4/1397—Processes of manufacture of electrodes based on inorganic compounds other than oxides or hydroxides, e.g. sulfides, selenides, tellurides, halogenides or LiCoFy
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10—Energy storage using batteries
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Inorganic Chemistry (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Battery Electrode And Active Subsutance (AREA)
  • Silicates, Zeolites, And Molecular Sieves (AREA)

Abstract

　本発明は、Ｍｎ、Ｆｅ、Ｃｏ及びＮｉからなる群から選択される少なくとも１つの遷移金属を含む遷移金属化合物、リチウム化合物、及び、ケイ素系高分子化合物の混合物を焼成して得られたリチウム遷移金属ケイ酸塩を二次電池の正極用材料として使用することを特徴とする。本発明のリチウム遷移金属ケイ酸塩は、遷移金属の単位量当たりのリチウムの吸蔵及び放出効率が高く、低コストであり、安定性及び安全性が高く、且つ、優れた充放電特性を有する二次電池を提供することができる。
PCT/JP2008/055749 2007-03-27 2008-03-26 二次電池用正極材料の製造方法 WO2008123311A1 (ja)

Priority Applications (3)

Application Number Priority Date Filing Date Title
US12/532,956 US8349217B2 (en) 2007-03-27 2008-03-26 Method for producing positive electrode material for secondary battery
EP08738937A EP2166600A4 (en) 2007-03-27 2008-03-26 METHOD FOR PRODUCING POSITIVE ELECTRODE MATERIAL FOR A SECONDARY BATTERY
JP2009509146A JPWO2008123311A1 (ja) 2007-03-27 2008-03-26 二次電池用正極材料の製造方法

Applications Claiming Priority (4)

Application Number Priority Date Filing Date Title
JP2007-082102 2007-03-27
JP2007082102 2007-03-27
JP2007-315091 2007-12-05
JP2007315091 2007-12-05

Publications (1)

Publication Number Publication Date
WO2008123311A1 true WO2008123311A1 (ja) 2008-10-16

Family

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Application Number Title Priority Date Filing Date
PCT/JP2008/055749 WO2008123311A1 (ja) 2007-03-27 2008-03-26 二次電池用正極材料の製造方法

Country Status (5)

Country Link
US (1) US8349217B2 (ja)
EP (1) EP2166600A4 (ja)
JP (1) JPWO2008123311A1 (ja)
KR (1) KR20090125268A (ja)
WO (1) WO2008123311A1 (ja)

Cited By (15)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2010108676A (ja) * 2008-10-29 2010-05-13 Toyota Central R&D Labs Inc 水系リチウム二次電池
JP2010225378A (ja) * 2009-03-23 2010-10-07 Toyota Central R&D Labs Inc リチウム二次電池
CN101521275B (zh) * 2009-04-07 2011-04-27 北京高盟新材料股份有限公司 一种二次锂离子电池正极材料硅酸镍锂的制备方法
JP2011187173A (ja) * 2010-03-04 2011-09-22 Toyota Central R&D Labs Inc 非水系二次電池用活物質及び非水系二次電池
JP2011249324A (ja) * 2010-04-28 2011-12-08 Semiconductor Energy Lab Co Ltd 蓄電装置用正極活物質、蓄電装置、及び電気推進車両、並びに蓄電装置の作製方法
US20120070708A1 (en) * 2009-05-22 2012-03-22 Koji Ohira Cathode active material, cathode and nonaqueous secondary battery
WO2012105039A1 (ja) * 2011-02-04 2012-08-09 株式会社日立製作所 リチウム二次電池用正極材料、リチウム二次電池用正極、及びリチウム二次電池
JP2012193088A (ja) * 2011-03-17 2012-10-11 Taiheiyo Cement Corp リチウムイオン電池用正極活物質の製造法
JP2012195134A (ja) * 2011-03-16 2012-10-11 Furukawa Electric Co Ltd:The リチウム遷移金属シリケート系正極活物質材料及び非水電解質２次電池用正極の製造方法
WO2014002602A1 (ja) * 2012-06-27 2014-01-03 Jnc株式会社 二次電池用負極活物質及びその製造方法、それを用いた負極並びにリチウムイオン電池
US9083046B2 (en) 2011-03-23 2015-07-14 Sharp Kabushiki Kaisha Cathode active material, cathode electrode and non-aqueous secondary battery
US9293234B2 (en) 2010-07-12 2016-03-22 Sharp Kabushiki Kaisha Positive electrode active material, positive electrode, and nonaqueous-electrolyte secondary battery
US9373844B2 (en) 2010-07-01 2016-06-21 Sharp Kabushiki Kaisha Positive electrode active substance containing lithium-containing metal oxide
US9379379B2 (en) 2011-09-05 2016-06-28 Shoei Chemical Inc. Cathode material for lithium ion secondary batteries, cathode member for lithium ion secondary batteries, lithium ion secondary battery, and method for producing cathode material for lithium ion secondary batteries
JP2020181653A (ja) * 2019-04-23 2020-11-05 国立大学法人 新潟大学 正極材の製造方法、正極材、及び、正極材を備えたリチウムイオン二次電池

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JP5298286B2 (ja) * 2009-02-04 2013-09-25 独立行政法人産業技術総合研究所 リチウムシリケート系化合物の製造方法
CN101920972B (zh) * 2010-06-28 2011-12-14 宁波大学 一种用于锂离子电池的硅酸钴锂正极材料的制备方法
JP5116177B2 (ja) 2010-06-28 2013-01-09 株式会社豊田自動織機 リチウムシリケート系化合物の製造方法
JP5917027B2 (ja) * 2010-06-30 2016-05-11 株式会社半導体エネルギー研究所 電極用材料の作製方法
JP5843766B2 (ja) * 2010-07-01 2016-01-13 シャープ株式会社 正極活物質、正極及び非水系二次電池
US9419271B2 (en) * 2010-07-02 2016-08-16 Semiconductor Energy Laboratory Co., Ltd. Electrode material and method for forming electrode material
KR20120039472A (ko) 2010-10-15 2012-04-25 가부시키가이샤 한도오따이 에네루기 켄큐쇼 축전 장치용 정극 활물질의 제작 방법
JP5698951B2 (ja) * 2010-10-19 2015-04-08 シャープ株式会社 正極活物質及びその製造方法、正極ならびに非水電解質二次電池
US9362560B2 (en) * 2011-03-08 2016-06-07 GM Global Technology Operations LLC Silicate cathode for use in lithium ion batteries
US9281515B2 (en) 2011-03-08 2016-03-08 Gholam-Abbas Nazri Lithium battery with silicon-based anode and silicate-based cathode
CN102219230B (zh) * 2011-05-17 2013-01-16 中南大学 锂离子电池正极材料硅酸亚铁锂的制备方法
KR101260685B1 (ko) * 2011-06-24 2013-05-10 한국과학기술연구원 리튬이온 이차전지용 전극 활물질 제조 방법 및 이를 이용한 리튬이온 이차전지
US9472805B2 (en) 2011-09-01 2016-10-18 Semiconductor Energy Laboratory Co., Ltd. Alkali metal silicate, alkali transition metal silicate, and method for synthesizing silicate
WO2014004789A2 (en) * 2012-06-27 2014-01-03 Precursor Energetics, Inc. Molecular precursors for synthesis of lithium-iron-containing cathode materials
WO2014010172A1 (ja) * 2012-07-10 2014-01-16 出光興産株式会社 硫化物系ガラスと硫化物系ガラスセラミックスの製造方法
CN103346300B (zh) * 2013-06-08 2015-12-09 合肥国轩高科动力能源有限公司 一种以稻壳粉为硅源原位合成硅酸盐/碳复合正极材料的方法
JP5769140B2 (ja) * 2014-01-30 2015-08-26 住友金属鉱山株式会社 リチウム二次電池用正極活物質の製造方法

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Cited By (26)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP2010108676A (ja) * 2008-10-29 2010-05-13 Toyota Central R&D Labs Inc 水系リチウム二次電池
JP2010225378A (ja) * 2009-03-23 2010-10-07 Toyota Central R&D Labs Inc リチウム二次電池
CN101521275B (zh) * 2009-04-07 2011-04-27 北京高盟新材料股份有限公司 一种二次锂离子电池正极材料硅酸镍锂的制备方法
US8999576B2 (en) * 2009-05-22 2015-04-07 Sharp Kabushiki Kaisha Cathode active material, cathode and nonaqueous secondary battery
US9419280B2 (en) 2009-05-22 2016-08-16 Sharp Kabushiki Kaisha Cathode active material, cathode and nonaqueous secondary battery
US20120070708A1 (en) * 2009-05-22 2012-03-22 Koji Ohira Cathode active material, cathode and nonaqueous secondary battery
US9350022B2 (en) 2009-05-22 2016-05-24 Sharp Kabushiki Kaisha Cathode active material, cathode and nonaqueous secondary battery
US9337489B2 (en) * 2009-05-22 2016-05-10 Sharp Kabushiki Kaisha Cathode active material, cathode and nonaqueous secondary battery
JP2011187173A (ja) * 2010-03-04 2011-09-22 Toyota Central R&D Labs Inc 非水系二次電池用活物質及び非水系二次電池
US10916774B2 (en) 2010-04-28 2021-02-09 Semiconductor Energy Laboratory Co., Ltd. Positive electrode active material of power storage device, power storage device, electrically propelled vehicle, and method for manufacturing power storage
US10224548B2 (en) 2010-04-28 2019-03-05 Semiconductor Energy Laboratory Co., Ltd. Positive electrode active material of power storage device, power storage device, electrically propelled vehicle, and method for manufacturing power storage
US9899678B2 (en) 2010-04-28 2018-02-20 Semiconductor Energy Laboratory Co., Ltd. Positive electrode active material of power storage device, power storage device, electrically propelled vehicle, and method for manufacturing power storage device
US9318741B2 (en) 2010-04-28 2016-04-19 Semiconductor Energy Laboratory Co., Ltd. Positive electrode active material of power storage device, power storage device, electrically propelled vehicle, and method for manufacturing power storage device
US12027702B2 (en) 2010-04-28 2024-07-02 Semiconductor Energy Laboratory Co., Ltd. Positive electrode active material of power storage device, power storage device, electrically propelled vehicle, and method for manufacturing power storage
JP2011249324A (ja) * 2010-04-28 2011-12-08 Semiconductor Energy Lab Co Ltd 蓄電装置用正極活物質、蓄電装置、及び電気推進車両、並びに蓄電装置の作製方法
US9373844B2 (en) 2010-07-01 2016-06-21 Sharp Kabushiki Kaisha Positive electrode active substance containing lithium-containing metal oxide
US9293234B2 (en) 2010-07-12 2016-03-22 Sharp Kabushiki Kaisha Positive electrode active material, positive electrode, and nonaqueous-electrolyte secondary battery
WO2012105039A1 (ja) * 2011-02-04 2012-08-09 株式会社日立製作所 リチウム二次電池用正極材料、リチウム二次電池用正極、及びリチウム二次電池
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