RU2019143348A - Клеевые композиции на основе растворителя - Google Patents
Клеевые композиции на основе растворителя Download PDFInfo
- Publication number
- RU2019143348A RU2019143348A RU2019143348A RU2019143348A RU2019143348A RU 2019143348 A RU2019143348 A RU 2019143348A RU 2019143348 A RU2019143348 A RU 2019143348A RU 2019143348 A RU2019143348 A RU 2019143348A RU 2019143348 A RU2019143348 A RU 2019143348A
- Authority
- RU
- Russia
- Prior art keywords
- solvent
- adhesive composition
- epoxy
- urethane resin
- resin mixture
- Prior art date
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- 239000000203 mixture Substances 0.000 title claims 19
- 239000002904 solvent Substances 0.000 title claims 12
- 239000000853 adhesive Substances 0.000 title claims 11
- 230000001070 adhesive effect Effects 0.000 title claims 11
- 229920000728 polyester Polymers 0.000 claims 16
- NBIIXXVUZAFLBC-UHFFFAOYSA-N Phosphoric acid Chemical compound OP(O)(O)=O NBIIXXVUZAFLBC-UHFFFAOYSA-N 0.000 claims 12
- 150000001875 compounds Chemical class 0.000 claims 8
- 239000011347 resin Substances 0.000 claims 8
- 229920005989 resin Polymers 0.000 claims 8
- 229920002803 thermoplastic polyurethane Polymers 0.000 claims 8
- 229910000147 aluminium phosphate Inorganic materials 0.000 claims 6
- 239000012948 isocyanate Substances 0.000 claims 4
- 239000004593 Epoxy Substances 0.000 claims 3
- -1 aliphatic isocyanate Chemical class 0.000 claims 3
- 239000004848 polyfunctional curative Substances 0.000 claims 3
- 125000000217 alkyl group Chemical group 0.000 claims 2
- 238000000034 method Methods 0.000 claims 2
- 239000007787 solid Substances 0.000 claims 2
- 239000002253 acid Substances 0.000 claims 1
- 239000007795 chemical reaction product Substances 0.000 claims 1
- 238000007865 diluting Methods 0.000 claims 1
- 238000010790 dilution Methods 0.000 claims 1
- 239000012895 dilution Substances 0.000 claims 1
- 150000002513 isocyanates Chemical class 0.000 claims 1
- 125000000962 organic group Chemical group 0.000 claims 1
- 229920005906 polyester polyol Polymers 0.000 claims 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
- C08G18/40—High-molecular-weight compounds
- C08G18/58—Epoxy resins
- C08G18/581—Reaction products of epoxy resins with less than equivalent amounts of compounds containing active hydrogen added before or during the reaction with the isocyanate component
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B15/00—Layered products comprising a layer of metal
- B32B15/04—Layered products comprising a layer of metal comprising metal as the main or only constituent of a layer, which is next to another layer of the same or of a different material
- B32B15/08—Layered products comprising a layer of metal comprising metal as the main or only constituent of a layer, which is next to another layer of the same or of a different material of synthetic resin
- B32B15/085—Layered products comprising a layer of metal comprising metal as the main or only constituent of a layer, which is next to another layer of the same or of a different material of synthetic resin comprising polyolefins
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B15/00—Layered products comprising a layer of metal
- B32B15/04—Layered products comprising a layer of metal comprising metal as the main or only constituent of a layer, which is next to another layer of the same or of a different material
- B32B15/08—Layered products comprising a layer of metal comprising metal as the main or only constituent of a layer, which is next to another layer of the same or of a different material of synthetic resin
- B32B15/09—Layered products comprising a layer of metal comprising metal as the main or only constituent of a layer, which is next to another layer of the same or of a different material of synthetic resin comprising polyesters
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B15/00—Layered products comprising a layer of metal
- B32B15/04—Layered products comprising a layer of metal comprising metal as the main or only constituent of a layer, which is next to another layer of the same or of a different material
- B32B15/08—Layered products comprising a layer of metal comprising metal as the main or only constituent of a layer, which is next to another layer of the same or of a different material of synthetic resin
- B32B15/095—Layered products comprising a layer of metal comprising metal as the main or only constituent of a layer, which is next to another layer of the same or of a different material of synthetic resin comprising polyurethanes
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B27/00—Layered products comprising a layer of synthetic resin
- B32B27/06—Layered products comprising a layer of synthetic resin as the main or only constituent of a layer, which is next to another layer of the same or of a different material
- B32B27/08—Layered products comprising a layer of synthetic resin as the main or only constituent of a layer, which is next to another layer of the same or of a different material of synthetic resin
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B27/00—Layered products comprising a layer of synthetic resin
- B32B27/32—Layered products comprising a layer of synthetic resin comprising polyolefins
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B27/00—Layered products comprising a layer of synthetic resin
- B32B27/36—Layered products comprising a layer of synthetic resin comprising polyesters
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B27/00—Layered products comprising a layer of synthetic resin
- B32B27/38—Layered products comprising a layer of synthetic resin comprising epoxy resins
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B27/00—Layered products comprising a layer of synthetic resin
- B32B27/40—Layered products comprising a layer of synthetic resin comprising polyurethanes
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B7/00—Layered products characterised by the relation between layers; Layered products characterised by the relative orientation of features between layers, or by the relative values of a measurable parameter between layers, i.e. products comprising layers having different physical, chemical or physicochemical properties; Layered products characterised by the interconnection of layers
- B32B7/04—Interconnection of layers
- B32B7/12—Interconnection of layers using interposed adhesives or interposed materials with bonding properties
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L75/00—Compositions of polyureas or polyurethanes; Compositions of derivatives of such polymers
- C08L75/04—Polyurethanes
- C08L75/06—Polyurethanes from polyesters
-
- C—CHEMISTRY; METALLURGY
- C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
- C09J—ADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
- C09J175/00—Adhesives based on polyureas or polyurethanes; Adhesives based on derivatives of such polymers
- C09J175/04—Polyurethanes
- C09J175/06—Polyurethanes from polyesters
-
- B—PERFORMING OPERATIONS; TRANSPORTING
- B32—LAYERED PRODUCTS
- B32B—LAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
- B32B2250/00—Layers arrangement
- B32B2250/02—2 layers
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G18/00—Polymeric products of isocyanates or isothiocyanates
- C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
- C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
- C08G18/30—Low-molecular-weight compounds
- C08G18/32—Polyhydroxy compounds; Polyamines; Hydroxyamines
- C08G18/3225—Polyamines
- C08G18/3228—Polyamines acyclic
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G63/00—Macromolecular compounds obtained by reactions forming a carboxylic ester link in the main chain of the macromolecule
- C08G63/02—Polyesters derived from hydroxycarboxylic acids or from polycarboxylic acids and polyhydroxy compounds
- C08G63/12—Polyesters derived from hydroxycarboxylic acids or from polycarboxylic acids and polyhydroxy compounds derived from polycarboxylic acids and polyhydroxy compounds
- C08G63/16—Dicarboxylic acids and dihydroxy compounds
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
- C08G63/00—Macromolecular compounds obtained by reactions forming a carboxylic ester link in the main chain of the macromolecule
- C08G63/91—Polymers modified by chemical after-treatment
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K3/00—Use of inorganic substances as compounding ingredients
- C08K3/32—Phosphorus-containing compounds
- C08K2003/329—Phosphorus containing acids
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K3/00—Use of inorganic substances as compounding ingredients
- C08K3/32—Phosphorus-containing compounds
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/04—Oxygen-containing compounds
- C08K5/06—Ethers; Acetals; Ketals; Ortho-esters
Landscapes
- Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Health & Medical Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Adhesives Or Adhesive Processes (AREA)
- Laminated Bodies (AREA)
- Epoxy Resins (AREA)
Claims (28)
1. Клеевая композиция на основе растворителя, содержащая:
(А) полиэфируретановую смолу;
(Б) сложное полиэфирное соединение с концевыми эпоксидными группами;
(В) фосфорную кислоту; и
(Г) алифатический изоцианатный отвердитель.
2. Клеевая композиция на основе растворителя по п. 1, отличающаяся тем, что полиэфируретановая смола представляет собой продукт реакции сложного полиэфирполиола и изоцианата.
3. Клеевая композиция на основе растворителя по п. 1, отличающаяся тем, что полиэфируретановая смола составляет от 65 до 99,5 мас.% от общей массы полиэфируретановой смолы (А), полиэфирного соединения с концевыми эпоксидными группами (Б) и фосфорной кислоты (В).
4. Клеевая композиция на основе растворителя по п. 1, отличающаяся тем, что полиэфирное соединение с концевыми эпоксидными группами составляет от 0,5 до 35 мас.% от общей массы полиэфируретановой смолы (А), полиэфирного соединения с концевыми эпоксидными группами (Б) и фосфорной кислоты (В).
5. Клеевая композиция на основе растворителя по п. 1, отличающаяся тем, что полиэфирное соединение с концевыми эпоксидными группами имеет структуру (I):
(I)
где, R1-имеет структуру (II):
(II)
где, G- имеет структуру (III):
(III)
где, J равен от 0 до 5, -R2- представляет собой двухвалентную органическую группу, R21-представляет собой двухвалентную алкильную группу, и -R22- представляет собой двухвалентную алкильную группу.
6. Клеевая композиция на основе растворителя по п. 1, отличающаяся тем, что фосфорная кислота составляет от 0,01 до 0,4 мас.% от общей массы полиэфируретановой смолы (А), полиэфирного соединения с концевыми эпоксидными группами (Б) и фосфорной кислоты (В).
7. Клеевая композиция на основе растворителя по п. 1, дополнительно содержащая растворитель.
8. Способ получения клеевой композиции на основе растворителя, включающий:
получение полиэфируретановой смолы;
получение полиэфирного соединения с концевыми эпоксидными группами;
смешивание полиэфируретановой смолы, полиэфирного соединения с концевыми эпоксидными группами и фосфорной кислоты с образованием смоляной смеси;
разбавление смоляной смеси растворителем с образованием разбавленной смоляной смеси с содержанием твердого вещества от 25 до 55 мас.% от общей массы разбавленной смоляной смеси; и
отверждение разбавленной смоляной смеси алифатическим изоцианатным отвердителем при соотношении компонентов смеси (массовых частей смоляной смеси до разбавления : массовых частей алифатического изоцианатного отвердителя) от 100:1 до 100:12.
9. Способ получения клеевой композиции на основе растворителя по п. 8, отличающийся тем, что разбавленная смоляная смесь характеризуется содержанием твердого вещества при нанесении от 35 до 40 процентов массовых от общей массы разбавленной смоляной смеси.
10. Многослойная структура, содержащая клеевую композицию по п.1.
Applications Claiming Priority (3)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| US201762517439P | 2017-06-09 | 2017-06-09 | |
| US62/517,439 | 2017-06-09 | ||
| PCT/US2018/028993 WO2018226320A1 (en) | 2017-06-09 | 2018-04-24 | Solvent-based adhesive compositions |
Publications (2)
| Publication Number | Publication Date |
|---|---|
| RU2019143348A true RU2019143348A (ru) | 2021-06-24 |
| RU2019143348A3 RU2019143348A3 (ru) | 2021-08-20 |
Family
ID=62152654
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| RU2019143348A RU2019143348A (ru) | 2017-06-09 | 2018-04-24 | Клеевые композиции на основе растворителя |
Country Status (9)
| Country | Link |
|---|---|
| US (1) | US11802227B2 (ru) |
| EP (1) | EP3635024B1 (ru) |
| JP (1) | JP7149293B2 (ru) |
| CN (1) | CN110691803B (ru) |
| AR (1) | AR111871A1 (ru) |
| MX (1) | MX2019014422A (ru) |
| RU (1) | RU2019143348A (ru) |
| TW (1) | TWI782019B (ru) |
| WO (1) | WO2018226320A1 (ru) |
Families Citing this family (4)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| AR119749A1 (es) * | 2019-07-12 | 2022-01-05 | Dow Global Technologies Llc | Composiciones a base de solvente |
| MX2022014031A (es) * | 2020-06-05 | 2022-12-02 | Dow Global Technologies Llc | Ester de fosfato de epoxi. |
| WO2023286644A1 (ja) * | 2021-07-16 | 2023-01-19 | 大日精化工業株式会社 | 接着剤 |
| CN114907812B (zh) * | 2022-06-21 | 2024-01-30 | 武汉弘毅共聚新材料科技有限公司 | 一种药物封装用低粘度vc胶及其制备方法与应用 |
Family Cites Families (20)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US4331782A (en) * | 1981-03-05 | 1982-05-25 | Ashland Oil, Inc. | Hydroxybenzoic acid-epoxy adduct capping agents for polyester resins |
| US4734303A (en) | 1985-07-19 | 1988-03-29 | Toyo Seikan Kaisha, Ltd. | Deep-draw-formed vessel and process for preparation thereof |
| US5096980A (en) * | 1988-06-28 | 1992-03-17 | Takeda Chemical Industries, Ltd. | Polyurethane adhesive of epoxy resin, polyisocyanate, phosphorus oxy acid, and carboxylic acid |
| US5202391A (en) | 1988-06-28 | 1993-04-13 | Takeda Chemical Industries, Ltd. | Polyurethane adhesive of epoxy resin, polyisocyanate, phosphorus oxy acid, and carboxylic acid |
| CA1336110C (en) * | 1989-02-03 | 1995-06-27 | Robert Gregory Swisher | Polymeric-containing compositions with improved oxidative stability |
| JPH0757386B2 (ja) | 1989-10-18 | 1995-06-21 | 東洋製罐株式会社 | 薄肉化絞り缶の製造方法 |
| JPH07108706B2 (ja) | 1991-11-12 | 1995-11-22 | 東洋製罐株式会社 | 薄肉化絞り缶の製造方法 |
| JPH07238270A (ja) * | 1994-02-25 | 1995-09-12 | Asahi Glass Co Ltd | フッ素樹脂の接着方法 |
| DE19781670T1 (de) | 1996-03-27 | 1999-04-08 | Toyo Kohan Co Ltd | Mit thermoplastischem Harz laminiertes Aluminiumlegierungsblech, Herstellungsverfahren und Herstellungsapparatur dafür |
| US6022913A (en) | 1996-09-06 | 2000-02-08 | Kureha Chemical Industry Co. Ltd. | Container for retort packaging, resin composition, and gas-barrier film prepared therefrom |
| EP0970987B1 (en) * | 1997-03-28 | 2003-10-22 | Asahi Glass Company Ltd. | Fluororesin films, laminate produced by using the same, and process for producing laminate |
| JP4457819B2 (ja) * | 2004-09-15 | 2010-04-28 | Ｊｆｅスチール株式会社 | 高耐食性表面処理鋼板及びその製造方法 |
| JP2006160904A (ja) | 2004-12-08 | 2006-06-22 | Toyo Mooton Kk | 接着剤組成物 |
| JP5194465B2 (ja) * | 2006-03-08 | 2013-05-08 | Ｊｆｅスチール株式会社 | 塗装鋼板、加工品および薄型テレビ用パネルならびに塗装鋼板の製造方法 |
| BRPI0815588A2 (pt) * | 2007-08-14 | 2015-02-18 | Momentive Performance Mat Inc | Compostos de poliorganossiloxano-poliuréia e/ou de poliorganossilo-xano-poliuretano |
| EP2468834A1 (de) * | 2010-12-23 | 2012-06-27 | Sika Technology AG | Hitzehärtende Dichtstoffzusammensetzungen mit schneller Hautbildung und hoher Zugfestigkeit |
| AR098270A1 (es) * | 2013-11-18 | 2016-05-18 | Rohm & Haas | Poliéster terminado en epoxi |
| AR098267A1 (es) | 2013-11-18 | 2016-05-18 | Rohm & Haas | Poliéster terminado en epoxi |
| AR098269A1 (es) * | 2013-11-18 | 2016-05-18 | Rohm & Haas | Poliéster terminado en epoxi |
| AR102914A1 (es) | 2014-11-12 | 2017-04-05 | Dow Global Technologies Llc | Adhesivo de laminación por embutición en frío de bisfenol-a-libre |
-
2018
- 2018-04-24 RU RU2019143348A patent/RU2019143348A/ru unknown
- 2018-04-24 CN CN201880035791.8A patent/CN110691803B/zh active Active
- 2018-04-24 US US16/620,805 patent/US11802227B2/en active Active
- 2018-04-24 EP EP18724394.4A patent/EP3635024B1/en active Active
- 2018-04-24 JP JP2019567569A patent/JP7149293B2/ja active Active
- 2018-04-24 MX MX2019014422A patent/MX2019014422A/es unknown
- 2018-04-24 WO PCT/US2018/028993 patent/WO2018226320A1/en active Application Filing
- 2018-05-15 AR ARP180101283A patent/AR111871A1/es active IP Right Grant
- 2018-05-16 TW TW107116539A patent/TWI782019B/zh active
Also Published As
| Publication number | Publication date |
|---|---|
| JP7149293B2 (ja) | 2022-10-06 |
| BR112019025112A2 (pt) | 2020-06-23 |
| US11802227B2 (en) | 2023-10-31 |
| CN110691803A (zh) | 2020-01-14 |
| TWI782019B (zh) | 2022-11-01 |
| TW201903109A (zh) | 2019-01-16 |
| EP3635024B1 (en) | 2022-10-26 |
| EP3635024A1 (en) | 2020-04-15 |
| JP2020523440A (ja) | 2020-08-06 |
| MX2019014422A (es) | 2020-02-05 |
| AR111871A1 (es) | 2019-08-28 |
| US20200199423A1 (en) | 2020-06-25 |
| WO2018226320A1 (en) | 2018-12-13 |
| RU2019143348A3 (ru) | 2021-08-20 |
| CN110691803B (zh) | 2022-06-24 |
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