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KR101881386B1 - 폴리머 블렌드를 포함하는 연료전지용 전해질 막, 및 이를 포함하는 막-전극 접합체 및 연료전지 - Google Patents

폴리머 블렌드를 포함하는 연료전지용 전해질 막, 및 이를 포함하는 막-전극 접합체 및 연료전지 Download PDF

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Publication number
KR101881386B1
KR101881386B1 KR1020150095424A KR20150095424A KR101881386B1 KR 101881386 B1 KR101881386 B1 KR 101881386B1 KR 1020150095424 A KR1020150095424 A KR 1020150095424A KR 20150095424 A KR20150095424 A KR 20150095424A KR 101881386 B1 KR101881386 B1 KR 101881386B1
Authority
KR
South Korea
Prior art keywords
fuel cell
membrane
same
polymer blend
electrod assembly
Prior art date
Application number
KR1020150095424A
Other languages
English (en)
Other versions
KR20170004708A (ko
Inventor
김형준
장종현
이소영
김보현
최선희
한종희
김진호
박종협
Original Assignee
한국과학기술연구원
율촌화학 주식회사
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by 한국과학기술연구원, 율촌화학 주식회사 filed Critical 한국과학기술연구원
Priority to KR1020150095424A priority Critical patent/KR101881386B1/ko
Priority to JP2016131572A priority patent/JP6259494B2/ja
Priority to US15/200,060 priority patent/US10305131B2/en
Publication of KR20170004708A publication Critical patent/KR20170004708A/ko
Application granted granted Critical
Publication of KR101881386B1 publication Critical patent/KR101881386B1/ko

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Classifications

    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1016Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018Polymeric electrolyte materials
    • H01M8/102Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1032Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having sulfur, e.g. sulfonated-polyethersulfones [S-PES]
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1016Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018Polymeric electrolyte materials
    • H01M8/102Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1027Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having carbon, oxygen and other atoms, e.g. sulfonated polyethersulfones [S-PES]
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G75/00Macromolecular compounds obtained by reactions forming a linkage containing sulfur with or without nitrogen, oxygen, or carbon in the main chain of the macromolecule
    • C08G75/20Polysulfones
    • C08G75/23Polyethersulfones
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/20Manufacture of shaped structures of ion-exchange resins
    • C08J5/22Films, membranes or diaphragms
    • C08J5/2206Films, membranes or diaphragms based on organic and/or inorganic macromolecular compounds
    • C08J5/2218Synthetic macromolecular compounds
    • C08J5/2256Synthetic macromolecular compounds based on macromolecular compounds obtained by reactions other than those involving carbon-to-carbon bonds, e.g. obtained by polycondensation
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1004Fuel cells with solid electrolytes characterised by membrane-electrode assemblies [MEA]
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1016Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018Polymeric electrolyte materials
    • H01M8/1041Polymer electrolyte composites, mixtures or blends
    • H01M8/1044Mixtures of polymers, of which at least one is ionically conductive
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M8/1016Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018Polymeric electrolyte materials
    • H01M8/1069Polymeric electrolyte materials characterised by the manufacturing processes
    • H01M8/1081Polymeric electrolyte materials characterised by the manufacturing processes starting from solutions, dispersions or slurries exclusively of polymers
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2381/00Characterised by the use of macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing sulfur with or without nitrogen, oxygen, or carbon only; Polysulfones; Derivatives of such polymers
    • C08J2381/06Polysulfones; Polyethersulfones
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2481/00Characterised by the use of macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing sulfur with or without nitrogen, oxygen, or carbon only; Polysulfones; Derivatives of such polymers
    • C08J2481/06Polysulfones; Polyethersulfones
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/10Fuel cells with solid electrolytes
    • H01M2008/1095Fuel cells with polymeric electrolytes
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00Electrolytes
    • H01M2300/0017Non-aqueous electrolytes
    • H01M2300/0065Solid electrolytes
    • H01M2300/0082Organic polymers
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30Hydrogen technology
    • Y02E60/50Fuel cells
    • Y02E60/521
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02PCLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50Manufacturing or production processes characterised by the final manufactured product

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Materials Engineering (AREA)
  • Composite Materials (AREA)
  • Dispersion Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Fuel Cell (AREA)
  • Conductive Materials (AREA)
  • Manufacture Of Macromolecular Shaped Articles (AREA)
  • Polyethers (AREA)
KR1020150095424A 2015-07-03 2015-07-03 폴리머 블렌드를 포함하는 연료전지용 전해질 막, 및 이를 포함하는 막-전극 접합체 및 연료전지 KR101881386B1 (ko)

Priority Applications (3)

Application Number Priority Date Filing Date Title
KR1020150095424A KR101881386B1 (ko) 2015-07-03 2015-07-03 폴리머 블렌드를 포함하는 연료전지용 전해질 막, 및 이를 포함하는 막-전극 접합체 및 연료전지
JP2016131572A JP6259494B2 (ja) 2015-07-03 2016-07-01 ポリマーブレンドを含む燃料電池用電解質膜及びこれを含む膜−電極接合体、並びに燃料電池
US15/200,060 US10305131B2 (en) 2015-07-03 2016-07-01 Electrolyte membrane for fuel cell comprising polymer blend, and membrane-electrode assembly and fuel cell comprising the same

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
KR1020150095424A KR101881386B1 (ko) 2015-07-03 2015-07-03 폴리머 블렌드를 포함하는 연료전지용 전해질 막, 및 이를 포함하는 막-전극 접합체 및 연료전지

Publications (2)

Publication Number Publication Date
KR20170004708A KR20170004708A (ko) 2017-01-11
KR101881386B1 true KR101881386B1 (ko) 2018-07-25

Family

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Family Applications (1)

Application Number Title Priority Date Filing Date
KR1020150095424A KR101881386B1 (ko) 2015-07-03 2015-07-03 폴리머 블렌드를 포함하는 연료전지용 전해질 막, 및 이를 포함하는 막-전극 접합체 및 연료전지

Country Status (3)

Country Link
US (1) US10305131B2 (ko)
JP (1) JP6259494B2 (ko)
KR (1) KR101881386B1 (ko)

Families Citing this family (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP6450980B2 (ja) * 2016-05-02 2019-01-16 本田技研工業株式会社 車両制御システム、車両制御方法、および車両制御プログラム
US20180286219A1 (en) * 2017-03-29 2018-10-04 Continental Automotive Systems, Inc. Customer Link
EP3655461A1 (en) * 2017-07-20 2020-05-27 Basf Se Sulfonated polyarylethersulfones and membranes thereof
WO2023161356A1 (en) * 2022-02-28 2023-08-31 Basf Se Process for the preparation of a membrane (m) containing a sulfonated polyarylenesulfone polymer (sp)

Family Cites Families (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP4001032B2 (ja) * 2003-02-28 2007-10-31 東ソー株式会社 ポリアリーレンエーテルスルホン系ブロック共重合体、その製造方法、並びにその用途
JP4807007B2 (ja) * 2005-08-25 2011-11-02 宇部興産株式会社 高分子電解質組成物およびその用途
EP2362473B1 (en) 2005-03-04 2012-10-24 Ube Industries, Ltd. Producion method for polymer electrolyte
JP4135728B2 (ja) * 2005-06-09 2008-08-20 東洋紡績株式会社 スルホン酸基含有ポリアリーレンエーテル系化合物およびその製造方法、該スルホン酸基含有ポリアリーレンエーテル系化合物を含有する樹脂組成物、高分子電解質膜、電解質膜/電極複合体、燃料電池および接着剤
EP1889863A4 (en) 2005-06-09 2010-03-17 Toyo Boseki SULFONIC ACID GROUP-MAIN POLYMER, METHOD OF MANUFACTURING THEREOF, RESIN COMPOSITION CONTAINING SUCH SULPHONIC ACID GROUP POLYMER, POLYMER ELECTROLYTE MEMBRANE, POLYMER ELECTROLYTE MEMBRANE / ELECTRODE ARRANGEMENT AND FUEL CELL
KR101344686B1 (ko) * 2011-03-18 2013-12-26 한국과학기술연구원 술폰화도가 상이한 고분자의 블렌드를 포함하는 연료전지 전해질막 및 이를 포함하는 막-전극 접합체 및 연료전지
KR101370806B1 (ko) * 2013-05-02 2014-03-12 한국과학기술연구원 히드록시기를 함유하는 술폰화 폴리에테르술폰 공중합체 및 그 제조방법, 연료전지용 고분자 전해질막 및 이를 포함하는 막 전극 접합체

Also Published As

Publication number Publication date
KR20170004708A (ko) 2017-01-11
JP2017017033A (ja) 2017-01-19
US20170005353A1 (en) 2017-01-05
JP6259494B2 (ja) 2018-01-10
US10305131B2 (en) 2019-05-28

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