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Mechanisms of optical limiting in fullerene-doped π-conjugated organic structures demonstrated with polyimide and COANP molecules

  • Molecular Spectroscopy
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Abstract

Possible mechanisms of optical limiting of visible radiation in conjugated organic structures based on polyimides and substituted pyridines sensitized with C60 and/or C70 fullerenes are studied using the Z-scan method. It is shown that reverse saturable absorption, two-photon absorption, and complex formation between the donor fragment of a π-conjugated molecule and fullerene contribute to the processes of nonlinear absorption. The absorption cross sections for excited states of the charge transfer complexes based on polyimide 6B-C70 and 2-cyclooctylamino-5-nitropyridine-C70 systems are calculated. The data obtained are quantitatively interpreted and compared with those provided by alternative methods.

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Authors and Affiliations

  1. Vavilov State Optical Institute, All-Russia Scientific Center, St. Petersburg, 199034, Russia

    N. V. Kamanina

  2. Institute of Automatics and Electrometry, Siberian Division, Russian Academy of Sciences, Novosibirsk, 630090, Russia

    A. I. Plekhanov

Authors
  1. N. V. Kamanina
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  2. A. I. Plekhanov
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__________

Translated from Optika i Spektroskopiya, Vol. 93, No. 3, 2002, pp. 443–452.

Original Russian Text Copyright © 2002 by Kamanina, Plekhanov.

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Kamanina, N.V., Plekhanov, A.I. Mechanisms of optical limiting in fullerene-doped π-conjugated organic structures demonstrated with polyimide and COANP molecules. Opt. Spectrosc. 93, 408–415 (2002). https://doi.org/10.1134/1.1509823

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  • DOI: https://doi.org/10.1134/1.1509823

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