Abstract
The cycle involving emission, atmospheric transport, chemical transformation and deposition, is often a major source of mercury contamination in places distant from anthropogenic sources. Therefore atmospheric modelling and simulation are important to evaluate the association between emissions and potential effects on human health. Unfortunately, once released into the atmosphere, mercury is subjected to a variety of complex physical-chemical processes before its deposition. Thus performing detailed mercury-cycle simulations on the large spatial scale required implies the use of parallel computing. In this work, chemistry, photolysis, emissions and deposition models have been linked to open-source atmospheric meteorological / dispersion software. The result is a parallel modelling system, capable of long term simulations and mercury emission reduction scenario analyses.
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Petersen, G., et al.: A comprehensive Eulerian modelling framework for airborne mercury species: model development and application in Europe. Atmospheric Environment 35-17, 3063–3074 (2001)
Berg, T., et al.: Atmospheric mercury species in the European Arctic: measurements and modelling. Atmospheric Environment 35(14), 2569–2582 (2001)
ATMET: ATmospheric Meteor. and Environmental Technologies: http://www.atmet.com
Walko, R.L., et al.: Coupled atmosphere-biophysics-hydrology models for environmental modeling. J. Appl. Meteor. 39, 931–944 (2000)
Pacyna, E., Pacyna, J.M., Pirrone, N.: Atmospheric Mercury Emissions in Europe from Anthropogenic Sources. Atmospheric Environment 35, 2987–2996 (2001)
Wild, O., Zhu, X., Prather, M.J.: Fast J: Accurate simulation of in- and below-cloud photolysis in tropospheric chemical models. J. Atmos. Chem. 37, 245–282 (2000)
Damian, V., Sandu, A., Damian, M., Potra, F., Carmichael, G.R.: The Kinetic Preprocessor KPP – A Software Environment for Solving Chemical Kinetics. Computers and Chemical Engineering 26(11), 1567–1579 (2002)
Pirrone, N., Mahaffey, K.R. (eds.): Dynamics of Mercury Pollution on Regional and Global Scales. Kluwer Academic, Dordrechet. Plenum Publishers (2004) (in Press)
Petersen, G., Iverfeldt, A., Munthe, J.: Atmospheric mercury species over central and northern Europe. Atmospheric Environment 29(1), 47–67 (1995)
Wesely, M.L., Hicks, B.B.: Some factors that affect the deposition of sulfur dioxide and similar gases on vegetation. Journ. of the Air Poll. Control Association, 1110–1116 (1977)
Slinn, S.A., Slinn, W.G.N.: Prediction for particle deposition on natural waters. Atomspheric Environment 14, 1013–1016 (1980)
Lindberg, S.E., et al.: Atmosphere-surface exchange of mercury in a forest: results of modeling and gradient approaches. Journ. of Geophys. Research 97, 2519–2528 (1992)
Xu, X., et al.: Formulation of bi-directional air-surface exchange of elemental mercury. Atmospheric Environment 33(27), 4345–4355 (1999)
Lindberg, S.E.: Forests and the global biogeochemical cycle of mercury: the importance of understanding air/vegetation exchange processes. In: Baeyens, W., et al. (eds.) Global and Regional Mercury Cycles: Sources, Fluxes, and Mass Balances, pp. 359–380. Kluwer, Dordrecht (1996)
Carpi, A., Lindberg, S.E.: Application of a Teflon dynamic flux chamber for quantifyng soil mercury flux: tests and results over background soil. Atmos. Env. 32(5), 873–882 (1998)
Munthe, J., et al.: Distribution of atmospheric mercury species in Northern Europe: final results from the MOE project. Atmospheric Environment 37 (2003)
Pirrone, N., et al.: Dynamic Processes of Mercury Over the Mediterranean Region. Atmospheric Environment 37 (2003)
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© 2005 Springer-Verlag Berlin Heidelberg
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Trunfio, G.A., Hedgecock, I.M., Pirrone, N. (2005). A Parallel Framework for the Simulation of Emission, Transport, Transformation and Deposition of Atmospheric Mercury on a Regional Scale. In: Gervasi, O., et al. Computational Science and Its Applications – ICCSA 2005. ICCSA 2005. Lecture Notes in Computer Science, vol 3480. Springer, Berlin, Heidelberg. https://doi.org/10.1007/11424758_110
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DOI: https://doi.org/10.1007/11424758_110
Publisher Name: Springer, Berlin, Heidelberg
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